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Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics￥Y. Zheng, H. Lin, T. Jiang, D. Zhu, S. Qi, W. Li, L. Li, D. Ji and W. Hu￥2022￥1616301X￥The disordered chain arrangement of polymer dielectrics has complex both internal and external effects on system performance, which generally stimulates the weak acquisition and grain boundaries of vapor-deposited organic small molecule films (VDOSMFs) with thermally activated charge transport. As a result, achieving "band-like" transmission of VDOSMs on polymer dielectrics is attempting to prove to be a major challenge. Three types of bi-polymer dielectrics are developed to modulate charge transport from thermally activated mode to "band-like" transport at the interfacial level. The bottom consisting of a polyimide layer is critical to interfacial modulation, which shows the selectively binding capability with up-dielectric layers to realize the modulation of charge transport, as corroborated by interface characterization and density functional-based tight-binding calculation. The findings provide an effective strategy for modulating the charge transport through polymer dielectric engineering and also recommend a podium to further comprehend the electrical characteristics of small molecules in organic thin-film transistors. 2022 Wiley-VCH GmbH.￥internal-pdf://1153944661/Modulating Charge Transport from Thermally Act.pdf￥10.1002/adfm.202211742￥https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/adfm.202211742?download=true￥ei 期刊论文
1616301X, 2022
作者:  Y. Zheng;  H. Lin;  T. Jiang;  D. Zhu;  S. Qi
收藏  |  浏览/下载：2/0  |  提交时间：2023/06/14
Modulating Charge Transport from Thermally Activated to "Band-Like" Through Interfacial Bottom-Up Binding Capability of Bilayer Polymer Dielectrics 期刊论文
1616301X, 2022
作者:  Y. Zheng;  H. Lin;  T. Jiang;  D. Zhu;  S. Qi
收藏  |  浏览/下载：5/0  |  提交时间：2023/07/17
Delicate crystallinity control enables high-efficiency P3HT organic photovoltaic cells 期刊论文
Journal of Materials Chemistry A, 2022, 卷号: 10, 期号: 7, 页码: 3418-3429
作者:  K. H. Xian;  Y. Liu;  J. W. Liu;  J. D. Yu;  Y. F. Xing
收藏  |  浏览/下载：7/0  |  提交时间：2023/06/14
Wafer-scale integration of stretchable semiconducting polymer microstructures via capillary gradient 期刊论文
NATURE COMMUNICATIONS, 1, 2021, 卷号: 12, 页码: 7038
作者:  Qiu, Yuchen;  Zhang, Bo;  Yang, Junchuan;  Gao, Hanfei;  Li S(李爽)
收藏  |  浏览/下载：16/0  |  提交时间：2022/10/25
Graphene assisting magnetic alignment of a high-performance semiconducting polymer for improved carrier transport 期刊论文
APPLIED PHYSICS LETTERS, 2020, 卷号: 117
作者:  Su, Songlin;  Pan, Guoxing;  Xiao, Xuhua;  Wang, Qi;  Zhang, Fapei
收藏  |  浏览/下载：19/0  |  提交时间：2020/10/26
Magnetic-field guided solvent vapor annealing for enhanced molecular alignment and carrier mobility of a semiconducting diketopyrrolopyrrole-based polymer 期刊论文
JOURNAL OF MATERIALS CHEMISTRY C, 2020, 卷号: 8
作者:  Xiao, Xuhua;  Pan, Guoxing;  Li, Tian;  Su, Songlin;  Zhu, Liangzheng
收藏  |  浏览/下载：31/0  |  提交时间：2020/11/26
Dopant-Dependent Increase in Seebeck Coefficient and Electrical Conductivity in Blended Polymers with Offset Carrier Energies 期刊论文
ADVANCED ELECTRONIC MATERIALS, 2019, 卷号: 5, 期号: 11
作者:  Li, Hui;  Plunkett, Evan;  Cai, Zhengxu;  Qiu, Botong;  Wei, Tianran
收藏  |  浏览/下载：86/0  |  提交时间：2019/12/31
Tailorable Metal-Ceramic (Cu-TiC0.5) Layered Electrode with High Mechanical Property and Conductivity 期刊论文
ACS APPLIED MATERIALS & INTERFACES, 2019, 卷号: 11, 期号: 47, 页码: 44413-44420
作者:  Si, Pengchao;  Duan, Chunyang;  Li, Mengqi;  Zhao, Zenghua;  Zhao, Dong
收藏  |  浏览/下载：62/0  |  提交时间：2020/03/24
Highly-soluble multi-alkylated polymer semiconductors and applications in high-performance field-effect transistors 期刊论文
JOURNAL OF MATERIALS CHEMISTRY C, 2019, 卷号: 7, 期号: 31, 页码: 9591-9598
作者:  Chen, Zhihui;  Huang, Jianyao;  Gao, Dong;  Yang, Jie;  Zhang, Weifeng
收藏  |  浏览/下载：65/0  |  提交时间：2019/09/30
Self-assembly diketopyrrolopyrrole-based materials and polymer blend with enhanced crystal alignment and property for organic field-effect transistors 期刊论文
ORGANIC ELECTRONICS, 2019, 卷号: 65, 页码: 96-99
作者:  Bi, Sheng;  Li, Yu;  He, Zhengran;  Ouyang, Zhongliang;  Guo, Qinglei
收藏  |  浏览/下载：9/0  |  提交时间：2019/12/02

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