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Reversible Three-Color Fluorescence Switching of an Organic Molecule in the Solid State via "PumpTrigger" Optical Manipulation¥R. Yang, X. Ren, L. Mei, G. Pan, X.-Z. Li, Z. Wu, S. Zhang, W. Ma, W. Yu, H.-H. Fang, C. Li, M.-Q. Zhu, Z. Hu, T. Sun, B. Xu and W. Tian¥2022¥Angewandte Chemie - International Edition¥14337851¥61¥20¥In photoswitches that undergo fluorescence switching upon ultraviolet irradiation, photoluminescence and photoisomerization often occur simultaneously, leading to unstable fluorescence properties. Here, we successfully demonstrated reversible solid-state triple fluorescence switching through "PumpTrigger" multiphoton manipulation. A novel fluorescence photoswitch, BOSA-SP, achieved green, yellow, and red fluorescence under excitation by pump light and isomerization induced by trigger light. The energy ranges of photoexcitation and photoisomerization did not overlap, enabling appropriate selection of the multiphoton light for "pump" and "trigger" photoswitching, respectively. Additionally, the large free volume of the spiropyran (SP) moiety in the solid state promoted reversible photoisomerization. Switching between "pump" and "trigger" light is useful for three-color tunable switching cell imaging, which can be exploited in programmable fluorescence switching. Furthermore, we exploited reversible dual-fluorescence switching in a single molecular system to successfully achieve two-color super-resolution imaging. 2022 Wiley-VCH GmbH.¥internal-pdf://0789088499/Reversible Three-Color Fluorescence Switching.pdf¥10.1002/anie.202117158¥https://onlinelibrary.wiley.com/doi/pdfdirect/10.1002/anie.202117158?download=true¥sci&ei
期刊论文
Angewandte Chemie - International Edition, 2022, 卷号: 61, 期号: 20
作者:
R. Yang
;
X. Ren
;
L. Mei
;
G. Pan
;
X.-Z. Li
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  |  
浏览/下载:18/0
  |  
提交时间:2023/06/14
Reversible Three-Color Fluorescence Switching of an Organic Molecule in the Solid State via "PumpTrigger" Optical Manipulation
期刊论文
Angewandte Chemie - International Edition, 2022, 卷号: 61, 期号: 20
作者:
R. Yang
;
X. Ren
;
L. Mei
;
G. Pan
;
X.-Z. Li
收藏
  |  
浏览/下载:7/0
  |  
提交时间:2023/07/17
Biosynthesis of a Phycocyanin Beta Subunit with Two Noncognate Chromophores in Escherichia coli
期刊论文
APPLIED BIOCHEMISTRY AND BIOTECHNOLOGY, 2020, 卷号: 191, 期号: 2, 页码: 763-771
作者:
Chen, Huaxin
;
Zheng, Caiyun
;
Jiang, Peng
;
Ji, Gengsheng
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  |  
浏览/下载:213/0
  |  
提交时间:2020/09/25
Phycobiliprotein
Phycocyanin
Lyase
Fluorescence
Chromophore
E
coli
Graphene Oxide Induced High Crystallinity of SAPO-11 Molecular Sieves for Improved Alkane Isomerization Performance
期刊论文
CHEMNANOMAT, 2019, 卷号: 5, 期号: 9, 页码: 1225
作者:
Du, Yanyan
;
Yao, Heliang
;
Zhao, Lei
;
Yang, Hongmei
;
Wang, Min
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  |  
浏览/下载:59/0
  |  
提交时间:2019/12/26
bifunctional catalysts
high crystallinity
graphene oxide
hydroisomerization
non-solvent method
Potential-Energy Surface and Dynamics Simulation of THBDBA: An Annulated Tetraphenylethene Derivative Combining Aggregation-Induced Emission and Switch Behavior
期刊论文
CHEMPHOTOCHEM, 2019, 卷号: 3, 期号: 9, 页码: 814-824
作者:
Ding, Wei-Lu
;
Peng, Xing-Liang
;
Cui, Gang-Long
;
Li, Ze-Sheng
;
Blancafort, Lluis
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  |  
浏览/下载:74/0
  |  
提交时间:2019/11/12
aggregation-induced emission
conical intersections
density functional calculations
dynamics simulations
photoswitches
Graphene Oxide Induced High Crystallinity of SAPO-11 Molecular Sieves for Improved Alkane Isomerization Performance
期刊论文
CHEMNANOMAT, 2019, 页码: 9
作者:
Du, Yanyan
;
Yao, Heliang
;
Zhao, Lei
;
Yang, Hongmei
;
Wang, Min
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  |  
浏览/下载:32/0
  |  
提交时间:2020/07/01
bifunctional catalysts
high crystallinity
graphene oxide
hydroisomerization
non-solvent method
Citric-acid-induced mesoporous SAPO-11 loaded with highly dispersed nickel for enhanced hydroisomerization of oleic acid to iso-alkanes
期刊论文
FUEL PROCESSING TECHNOLOGY, 2019, 卷号: 187, 页码: 52-62
作者:
Yang, Lingmei
;
Xing, Shiyou
;
Sun, Hongzhe
;
Miao, Changlin
;
Li, Ming
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  |  
浏览/下载:37/0
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提交时间:2020/10/29
Citric acid
Highly dispersed Ni
Mesoporous SAPO-11
Hydroisomerization
Oleic acid
Visible-Light-Induced Organic Photochemical Reactions through Energy-Transfer Pathways.
期刊论文
Angewandte Chemie (International ed. in English), 2019, 卷号: 58, 期号: 6, 页码: 1586-1604
作者:
Zhou, Quan-Quan
;
Zou, You-Quan
;
Lu, Liang-Qiu*
;
Xiao, Wen-Jing*
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  |  
浏览/下载:4/0
  |  
提交时间:2019/12/23
cycloaddition
energy transfer
isomerization
photocatalysis
photosensitization
Dissociation of [HCCH](2+) to H-2(+) and C-2(+): a benchmark reaction involving H migration, H-H combination, and C-H bond cleavage
期刊论文
PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2018, 卷号: 20, 页码: 27725-27729
作者:
Xu, Shenyue
;
Zhao, Hongyan
;
Zhu, Xiaolong
;
Guo, Dalong
;
Feng, Wentian
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  |  
浏览/下载:31/0
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提交时间:2019/03/27
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