Third-order nonlinear optical properties of GeS2-Sb2S3-CdS chalcogenide glasses
Guo, Haitao; Hou, Chaoqi; Gao, Fei; Lin, Aoxiang; Wang, Pengfei; Zhou, Zhiguang; Lu, Min; Wei, Wei; Peng, Bo
刊名optics express
2010-10-25
卷号18期号:22页码:23275-23284
英文摘要the third-order nonlinear optical properties of ges2-sb2s3-cds chalcogenide glasses were investigated utilizing the z-scan and femtosecond time-resolved optical kerr effect (oke) methods at the wavelength of 800nm, respectively. the compositional dependences were analyzed and the influencing factors including the linear refractive index, the concentration of lone electron pairs, the optical bandgap and the amount of weak covalent/ homopolar bonds were discussed. a glass, i.e. 76ges(2)center dot 19sb(2)s(3 center dot)5cds, with large nonlinear refrative index (n(2) = 5.63 x 10(-14) cm(2)/w), low nonlinear absorption coefficient (beta = 0.88 cm/gw) and minimum figure of merit (fom = 2 beta lambda/n(2) = 2.51) was finally prepared. the electronic contribution in weak heterpolar covalent and homopolar bonds are responsible for large n(2) in chalcogenide glass, and the sheik-bahae rule combining the moss rule are proved to be an effective guidance for estimating the third-order nonlinearities and further optimizing the compositions in chalcogenide glasses. (c) 2010 optical society of america
WOS标题词science & technology ; physical sciences
类目[WOS]optics
研究领域[WOS]optics
关键词[WOS]as-s-se ; system ; fibers
收录类别SCI ; EI
语种英语
WOS记录号WOS:000283560400068
公开日期2015-09-15
内容类型期刊论文
源URL[http://ir.opt.ac.cn/handle/181661/25290]  
专题西安光学精密机械研究所_先进光电与生物材料研发中心
作者单位Chinese Acad Sci, Xian Inst Opt & Precis Mech, State Key Lab Transient Opt & Photon, Xian 710119, Shanxi, Peoples R China
推荐引用方式
GB/T 7714
Guo, Haitao,Hou, Chaoqi,Gao, Fei,et al. Third-order nonlinear optical properties of GeS2-Sb2S3-CdS chalcogenide glasses[J]. optics express,2010,18(22):23275-23284.
APA Guo, Haitao.,Hou, Chaoqi.,Gao, Fei.,Lin, Aoxiang.,Wang, Pengfei.,...&Peng, Bo.(2010).Third-order nonlinear optical properties of GeS2-Sb2S3-CdS chalcogenide glasses.optics express,18(22),23275-23284.
MLA Guo, Haitao,et al."Third-order nonlinear optical properties of GeS2-Sb2S3-CdS chalcogenide glasses".optics express 18.22(2010):23275-23284.
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