Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies

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	Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies
	Niziolek, Alexander M.1; Onel, Onur 1; Elia, Josephine A.1; Baliban, Richard C.1; Xiao, Xin 2; Floudas, Christodoulos A.1
刊名	INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
	2014-11-05
卷号	53 期号:44 页码:17002-17025
关键词	NATURAL-GAS PROCESSES SWINE WASTE-WATER LEMNA-MINOR CHEMICAL-PROCESSES TROPSCH SYNTHESIS DUCKWEED BIOMASS GROWING DUCKWEED DIMETHYL ETHER HYBRID BIOMASS CO2 EMISSION
ISSN号	0888-5885
其他题名	Ind. Eng. Chem. Res.
中文摘要	The thermochemical conversion of coal and biomass to liquid transportation fuels from a synthesis gas intermediate is investigated using an optimization-based process synthesis framework. Two distinct types of coal (LV bituminous and coal commonly found in the province of Anhui, China) and two types of biomass (hardwood and duckweed) are considered as feedstocks. The superstructure incorporates alternative conversion pathways of synthesis gas which include methanol formation and conversion into FischerTropsch hydrocarbons. Methanol may be converted to gasoline or olefins, and the olefins may be subsequently converted to gasoline and distillate. A rigorous deterministic global optimization branch-and-bound framework is utilized to determine the optimal process topology that produces liquid fuels at the lowest possible cost. Economies of scale are evident as the refinery capacity increases and it is observed that the fuel ratios of the final liquid products have a significant impact on the optimal topology of the plant. The results suggest that liquid fuels production from coal and biomass can be competitive with petroleum-based processes.
英文摘要	The thermochemical conversion of coal and biomass to liquid transportation fuels from a synthesis gas intermediate is investigated using an optimization-based process synthesis framework. Two distinct types of coal (LV bituminous and coal commonly found in the province of Anhui, China) and two types of biomass (hardwood and duckweed) are considered as feedstocks. The superstructure incorporates alternative conversion pathways of synthesis gas which include methanol formation and conversion into FischerTropsch hydrocarbons. Methanol may be converted to gasoline or olefins, and the olefins may be subsequently converted to gasoline and distillate. A rigorous deterministic global optimization branch-and-bound framework is utilized to determine the optimal process topology that produces liquid fuels at the lowest possible cost. Economies of scale are evident as the refinery capacity increases and it is observed that the fuel ratios of the final liquid products have a significant impact on the optimal topology of the plant. The results suggest that liquid fuels production from coal and biomass can be competitive with petroleum-based processes.
WOS标题词	Science & Technology ; Technology
类目[WOS]	Engineering, Chemical
研究领域[WOS]	Engineering
关键词[WOS]	NATURAL-GAS PROCESSES ; SWINE WASTE-WATER ; LEMNA-MINOR ; CHEMICAL-PROCESSES ; TROPSCH SYNTHESIS ; DUCKWEED BIOMASS ; GROWING DUCKWEED ; DIMETHYL ETHER ; HYBRID BIOMASS ; CO2 EMISSION
收录类别	SCI
原文出处	://WOS:000344516900010
语种	英语
WOS记录号	WOS:000344516900010
公开日期	2015-04-01
内容类型	期刊论文
源URL	[http://ir.ipe.ac.cn/handle/122111/11811]
专题	过程工程研究所_研究所（批量导入）
作者单位	1.Princeton Univ, Dept Chem & Biol Engn, Princeton, NJ 08544 USA 2.Chinese Acad Sci, Langfang Engn & Technol Ctr, Natl Engn Lab Hydromet Cleaner Prod Technol, Inst Proc Engn, Beijing 100190, Peoples R China
推荐引用方式 GB/T 7714	Niziolek, Alexander M.,Onel, Onur,Elia, Josephine A.,et al. Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2014,53(44):17002-17025.
APA	Niziolek, Alexander M.,Onel, Onur,Elia, Josephine A.,Baliban, Richard C.,Xiao, Xin,&Floudas, Christodoulos A..(2014).Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,53(44),17002-17025.
MLA	Niziolek, Alexander M.,et al."Coal and Biomass to Liquid Transportation Fuels: Process Synthesis and Global Optimization Strategies".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 53.44(2014):17002-17025.