Facile synthesis of phosphorus doped graphitic carbon nitride polymers with enhanced visible-light photocatalytic activity | |
Zhang, L. ; Chen, X. ; Guan, J ; Jiang, Y ; Hou, T ; Mu, X. | |
刊名 | Materials Research Bulletin
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2013 | |
卷号 | 48期号:9页码:3485-3491 |
关键词 | A. Nitrides A. Polymers A. Semiconductors D. Catalytic properties D. Optical properties |
中文摘要 | Phosphorus-doped carbon nitride materials were prepared by a one-pot green synthetic approach using dicyandiamide monomer and a phosphorus containing ionic liquid as precursors. The as-prepared materials were subjected to several characterizations and investigated as metal-free photocatalysts for the degradation of organic pollutants (dyes like Rhodamine B, Methyl orange) in aqueous solution under visible light. Results revealed that phosphorus-doped carbon nitride have a higher photocatalytic activity for decomposing Rhodamine B and Methyl orange in aqueous solution than undoped g-C3N4, which was attributed to the favorable textural, optical and electronic properties caused by doping with phosphorus heteroatoms into carbon nitride host. A facile postannealing treatment further improved the activity of the photocatalytic system, due to the higher surface area and smaller structural size in the postcalcined catalysts. The phosphorus-doped carbon nitride showed high visible-light photocatalytic activity, making them promising materials for a wide range of potential applications in photochemistry. |
学科主题 | 绿色化学催化 |
收录类别 | SCI |
语种 | 英语 |
公开日期 | 2014-03-21 |
内容类型 | 期刊论文 |
源URL | [http://ir.qibebt.ac.cn:8080/handle/337004/1636] ![]() |
专题 | 青岛生物能源与过程研究所_绿色化学催化团队 |
推荐引用方式 GB/T 7714 | Zhang, L.,Chen, X.,Guan, J,et al. Facile synthesis of phosphorus doped graphitic carbon nitride polymers with enhanced visible-light photocatalytic activity[J]. Materials Research Bulletin,2013,48(9):3485-3491. |
APA | Zhang, L.,Chen, X.,Guan, J,Jiang, Y,Hou, T,&Mu, X..(2013).Facile synthesis of phosphorus doped graphitic carbon nitride polymers with enhanced visible-light photocatalytic activity.Materials Research Bulletin,48(9),3485-3491. |
MLA | Zhang, L.,et al."Facile synthesis of phosphorus doped graphitic carbon nitride polymers with enhanced visible-light photocatalytic activity".Materials Research Bulletin 48.9(2013):3485-3491. |
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