Low-temperature selective oxidation of methane to ethane and ethylene over BaCO3/La2O3 catalysts prepared by urea combustion method
Yang J(杨建); Zhao J(赵军); Song HL(宋焕玲); Chou LJ(丑凌军)
刊名Catalysis Communications
2005
卷号7页码:59-63
关键词Low-temperature Oxidative coupling of methane BaCO3/La2O3 catalyst Urea combustion method Hot spot
ISSN号1566-7367
通讯作者李树本
中文摘要A series of BaCO3/La2O3 catalysts have been prepared using urea combustion method, and tested their activity in oxidative conversion of methane to ethane and ethylene below 600 ℃. For 5% BaCO3/La2O3 catalyst, under integral conditions, CH4 conversion of 31.8% with C2 selectivity of 45.9% have been obtained at 320 ℃. With the increase of BaCO3 contents, CH4 conversion and C2 selectivity are improved. The temperature profiles of reactor have been described and found that the distribution of hot spots on catalyst bed is related to the low-temperature activity of catalyst.
收录类别SCI
资助信息the Ministry of Science and Technology of China (Grant 1999022406);Nature Science Foundation of China (Grant 20378081)
语种英语
WOS记录号WOS:000234993600001
公开日期2014-01-10
内容类型期刊论文
源URL[http://210.77.64.217/handle/362003/5029]  
专题兰州化学物理研究所_OSSO国家重点实验室
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Yang J,Zhao J,Song HL,et al. Low-temperature selective oxidation of methane to ethane and ethylene over BaCO3/La2O3 catalysts prepared by urea combustion method[J]. Catalysis Communications,2005,7:59-63.
APA Yang J,Zhao J,Song HL,&Chou LJ.(2005).Low-temperature selective oxidation of methane to ethane and ethylene over BaCO3/La2O3 catalysts prepared by urea combustion method.Catalysis Communications,7,59-63.
MLA Yang J,et al."Low-temperature selective oxidation of methane to ethane and ethylene over BaCO3/La2O3 catalysts prepared by urea combustion method".Catalysis Communications 7(2005):59-63.
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