Prolonging exciton lifetime of WSe2 monolayer through image dipole interaction leading to huge enhancement of photocurrent
K. J. Lee; J. P. So; S. K. Chamoli; H. C. Lee; H. G. Park and M. H. Cho
刊名Nanophotonics
2023
页码9
ISSN号2192-8606
DOI10.1515/nanoph-2022-0590
英文摘要Two-dimensional transition metal dichalcogenides (2D TMDs) have been demonstrated as one of the most outstanding materials not only for fundamental science but also for a wide range of photonic applications. However, an efficient way to control their excitonic properties is still needed for advanced applications with superior device performance. Here, we show that the exciton lifetime of WSe2 monolayer can be prolonged using metamaterials. We observe a similar to 100% reduction in the electron-hole recombination rate of WSe2 monolayer placed on a hyperbolic metamaterial substrate and demonstrate that such a remarkable change results from the destructive image dipole interaction with the in-plane exciton transition dipole. Furthermore, this substantial increase in exciton lifetime leads to order-of-magnitude (10-fold) enhancement of photocurrent in the 2D WSe2-based hybrid photodetector with metamaterials. Tailoring the optical transition properties of 2D TMD materials with specially designed metamaterials, demonstrated here, will pave the way for developing 2D material-based optoelectronics.
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语种英语
内容类型期刊论文
源URL[http://ir.ciomp.ac.cn/handle/181722/67591]  
专题中国科学院长春光学精密机械与物理研究所
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K. J. Lee,J. P. So,S. K. Chamoli,et al. Prolonging exciton lifetime of WSe2 monolayer through image dipole interaction leading to huge enhancement of photocurrent[J]. Nanophotonics,2023:9.
APA K. J. Lee,J. P. So,S. K. Chamoli,H. C. Lee,&H. G. Park and M. H. Cho.(2023).Prolonging exciton lifetime of WSe2 monolayer through image dipole interaction leading to huge enhancement of photocurrent.Nanophotonics,9.
MLA K. J. Lee,et al."Prolonging exciton lifetime of WSe2 monolayer through image dipole interaction leading to huge enhancement of photocurrent".Nanophotonics (2023):9.
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