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Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts
Wang, Yanping2; Sun, Xiaofeng1; Xian, Tao1; Liu, Guorong2; Yang, Hua2
刊名OPTICAL MATERIALS
2021
卷号113
关键词BaTiO3 particles Bi2WO6 hierarchical architectures BaTiO3/Bi2WO6 heterojunctions Photodegradation Simulated dye wastewater
ISSN号0925-3467
DOI10.1016/j.optmat.2021.110853
英文摘要To reveal the photodegradation process of mixture dye solutions in different pH environments by photocatalysts is a key point to promote the practical application of potocatalysis technology in purifying industrial dye wastewater. Herein we report the photocatalytic degradation of various organic dyes (MO, RhB, MB) and MO/RhB/MB mixture solutions in different pH environments by using novel BaTiO3/Bi2WO6 (BTO/BWO) heterojunction composites as the photocatalyst and simulated sunlight as the light source. The BTO/BWO heterojunction photocatalysts were prepared by immobilizing BTO particles onto rose flower-like BWO hierarchical architectures. Among the as-derived samples, the 15 wt%BTO/BWO composite is determined to have the highest photodegradation performance, which is ascribed to the efficient separation of photoexcited electron/hole pairs due to the Z-scheme electron transfer mechanism. The photodegradation of the dyes is found to be highly dependent on the acidic-alkaline environments. Moreover, an interesting competitive photodegradation phenomenon between the dyes is observed in the MO/RhB/MB mixture solutions. Superoxide (center dot O-2(-)) and hydroxyl (center dot OH) radicals are suggested to be the direct reactive species causing the dye photodegradation in the present photocatalytic system.
WOS研究方向Materials Science ; Optics
语种英语
出版者ELSEVIER
WOS记录号WOS:000633031700001
内容类型期刊论文
源URL[http://ir.lut.edu.cn/handle/2XXMBERH/148343]  
专题理学院
作者单位1.Qinghai Normal Univ, Coll Phys & Elect Informat Engn, Xining 810008, Peoples R China
2.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Peoples R China;
推荐引用方式
GB/T 7714
Wang, Yanping,Sun, Xiaofeng,Xian, Tao,et al. Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts[J]. OPTICAL MATERIALS,2021,113.
APA Wang, Yanping,Sun, Xiaofeng,Xian, Tao,Liu, Guorong,&Yang, Hua.(2021).Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts.OPTICAL MATERIALS,113.
MLA Wang, Yanping,et al."Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts".OPTICAL MATERIALS 113(2021).
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