Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts | |
Wang, Yanping2; Sun, Xiaofeng1; Xian, Tao1; Liu, Guorong2; Yang, Hua2 | |
刊名 | OPTICAL MATERIALS
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2021 | |
卷号 | 113 |
关键词 | BaTiO3 particles Bi2WO6 hierarchical architectures BaTiO3/Bi2WO6 heterojunctions Photodegradation Simulated dye wastewater |
ISSN号 | 0925-3467 |
DOI | 10.1016/j.optmat.2021.110853 |
英文摘要 | To reveal the photodegradation process of mixture dye solutions in different pH environments by photocatalysts is a key point to promote the practical application of potocatalysis technology in purifying industrial dye wastewater. Herein we report the photocatalytic degradation of various organic dyes (MO, RhB, MB) and MO/RhB/MB mixture solutions in different pH environments by using novel BaTiO3/Bi2WO6 (BTO/BWO) heterojunction composites as the photocatalyst and simulated sunlight as the light source. The BTO/BWO heterojunction photocatalysts were prepared by immobilizing BTO particles onto rose flower-like BWO hierarchical architectures. Among the as-derived samples, the 15 wt%BTO/BWO composite is determined to have the highest photodegradation performance, which is ascribed to the efficient separation of photoexcited electron/hole pairs due to the Z-scheme electron transfer mechanism. The photodegradation of the dyes is found to be highly dependent on the acidic-alkaline environments. Moreover, an interesting competitive photodegradation phenomenon between the dyes is observed in the MO/RhB/MB mixture solutions. Superoxide (center dot O-2(-)) and hydroxyl (center dot OH) radicals are suggested to be the direct reactive species causing the dye photodegradation in the present photocatalytic system. |
WOS研究方向 | Materials Science ; Optics |
语种 | 英语 |
出版者 | ELSEVIER |
WOS记录号 | WOS:000633031700001 |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/148343] ![]() |
专题 | 理学院 |
作者单位 | 1.Qinghai Normal Univ, Coll Phys & Elect Informat Engn, Xining 810008, Peoples R China 2.Lanzhou Univ Technol, State Key Lab Adv Proc & Recycling Nonferrous Met, Lanzhou 730050, Peoples R China; |
推荐引用方式 GB/T 7714 | Wang, Yanping,Sun, Xiaofeng,Xian, Tao,et al. Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts[J]. OPTICAL MATERIALS,2021,113. |
APA | Wang, Yanping,Sun, Xiaofeng,Xian, Tao,Liu, Guorong,&Yang, Hua.(2021).Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts.OPTICAL MATERIALS,113. |
MLA | Wang, Yanping,et al."Photocatalytic purification of simulated dye wastewater in different pH environments by using BaTiO3/Bi2WO6 heterojunction photocatalysts".OPTICAL MATERIALS 113(2021). |
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