Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation | |
Zhang, Ting; Liu, Jin; Chen, Minmin; Wang, Yi | |
刊名 | DESALINATION AND WATER TREATMENT |
2018-03 | |
卷号 | 107页码:91-99 |
关键词 | Attapulgite (ATP) Heterogeneous Fenton catalyst Degradation HA-Na |
ISSN号 | 1944-3994 |
DOI | 10.5004/dwt.2018.22111 |
英文摘要 | A novel heterogeneous Fenton catalyst Fe/organo-attapulgite (Fe/OATP) was prepared by introducing nano-Fe into organic modified attapulgite with redox method. The new catalyst was characterized by XRD, IR and SEM, and a series of experiments were conducted for investigating the influences of pH value, catalyst dosage, hydrogen peroxide concentration, reaction temperature and initial concentration of HA-Na solution on the degradation ratios of HA-Na in Fe/OATP/H2O2 heterogeneous Fenton system. Through a number of degradation experiments under various conditions, the results showed that the removal ratio of HA-Na can reach more than 97% at the condition of pH value 8, the reaction temperature 70 degrees C, the initial HA-Na concentration 100 mg/L, the catalysts dosage 10 g/L, and the H2O2 concentration 78.4 mmol/L. According to the results of dynamics experiments, the degradation of HA-Na followed the first-order kinetics. Fe/OATP catalyst has a wide pH range in heterogeneous Fenton reaction and can be reused for many runs with good capacity of HA-Na degradation. |
资助项目 | National Natural Science Foundation of China[51302123] |
WOS研究方向 | Engineering ; Water Resources |
语种 | 英语 |
出版者 | DESALINATION PUBL |
WOS记录号 | WOS:000445119300010 |
状态 | 已发表 |
内容类型 | 期刊论文 |
源URL | [http://119.78.100.223/handle/2XXMBERH/32753] |
专题 | 石油化工学院 |
通讯作者 | Zhang, Ting |
作者单位 | Lanzhou Univ Technol, Dept Petrochem Engn, Lanzhou 730050, Gansu, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Ting,Liu, Jin,Chen, Minmin,et al. Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation[J]. DESALINATION AND WATER TREATMENT,2018,107:91-99. |
APA | Zhang, Ting,Liu, Jin,Chen, Minmin,&Wang, Yi.(2018).Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation.DESALINATION AND WATER TREATMENT,107,91-99. |
MLA | Zhang, Ting,et al."Preparation of heterogeneous Fenton catalyst Fe/organo-attapulgite and its performance in sodium humate degradation".DESALINATION AND WATER TREATMENT 107(2018):91-99. |
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