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Short-Time Hydrothermal Synthesis of CuBi2O4 Nanocolumn Arrays for Efficient Visible-Light Photocatalysis
Wang, Yi1; Cai, Fang1,2; Guo, Pengran2; Lei, Yongqian2; Xi, Qiaoyue2; Wang, Fuxian2
刊名NANOMATERIALS
2019-09
卷号9期号:9
关键词CuBi2O4 short-time hydrothermal method photocatalytic degradation methylene blue
DOI10.3390/nano9091257
英文摘要In this article, a short-time hydrothermal method is developed to prepare CuBi2O4 nanocolumn arrays. By using Bi(NO3)(3)?5H(2)O in acetic acid and Cu(NO3)(2)?3H(2)O in ethanol as precursor solutions, tetragonal CuBi2O4 with good visible light absorption can be fabricated within 0.5 h at 120 degrees C. Tetragonal structured CuBi2O4 can be formed after 15 min hydrothermal treatment, however it possesses poor visible light absorption and low photocatalytic activity. Extending the hydrothermal treatment duration to 0.5 h results in a significant improvement invisible light absorption of the tetragonal CuBi2O4. The CuBi2O4 obtained through 0.5 h hydrothermal synthesis shows a band gap of 1.75 eV and exhibits the highest photocatalytic performance among the CuBi2O4 prepared with various hydrothermal time. The removal rate of methylene blue by the 0.5 h CuBi2O4 reaches 91% under visible light irradiation for 0.5 h. This study proposes a novel strategy to prepare photoactive CuBi2O4 nanocolumn arrays within 0.5 h at a moderate temperature of 120 degrees C. The hydrothermal method provides a facile strategy for the fast synthesis of metal-oxide-based photocatalysts at mild reaction conditions.
资助项目National Natural Science Foundation of China[61904167][51562023][21707128] ; Funding of Guangdong Provincial Key Laboratory of Emergency Test for Dangerous Chemicals[KF2018001]
WOS研究方向Science & Technology - Other Topics ; Materials Science
语种英语
出版者MDPI
WOS记录号WOS:000489101900074
状态已发表
内容类型期刊论文
源URL[http://119.78.100.223/handle/2XXMBERH/31600]  
专题石油化工学院
通讯作者Xi, Qiaoyue; Wang, Fuxian
作者单位1.Lanzhou Univ Technol, Coll Petrochem Technol, Lanzhou 730050, Gansu, Peoples R China
2.Guangdong Inst Anal, Guangdong Engn Technol Res Ctr Line Monitoring Wa, Guangdong Prov Key Lab Emergency Test Dangerous C, Guangzhou 510070, Guangdong, Peoples R China
推荐引用方式
GB/T 7714
Wang, Yi,Cai, Fang,Guo, Pengran,et al. Short-Time Hydrothermal Synthesis of CuBi2O4 Nanocolumn Arrays for Efficient Visible-Light Photocatalysis[J]. NANOMATERIALS,2019,9(9).
APA Wang, Yi,Cai, Fang,Guo, Pengran,Lei, Yongqian,Xi, Qiaoyue,&Wang, Fuxian.(2019).Short-Time Hydrothermal Synthesis of CuBi2O4 Nanocolumn Arrays for Efficient Visible-Light Photocatalysis.NANOMATERIALS,9(9).
MLA Wang, Yi,et al."Short-Time Hydrothermal Synthesis of CuBi2O4 Nanocolumn Arrays for Efficient Visible-Light Photocatalysis".NANOMATERIALS 9.9(2019).
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