Photocatalytic degradation activity of BaTiO3 nanoparticles modified with au in simulated sunlight | |
Xian, Tao1; Di, Lijing1,2; Ma, Jun1; Sang, Cuicui1; Wei, Xuegang1; Zhou, Yongjie1 | |
刊名 | Cailiao Yanjiu Xuebao/Chinese Journal of Materials Research |
2017-02-25 | |
卷号 | 31期号:2页码:102-109 |
关键词 | Aromatic compounds Barium titanate Complexation Deposition Gold Gold deposits High resolution transmission electron microscopy Nanoparticles Photocatalysis Photocatalytic activity Photoluminescence spectroscopy Reusability Surface plasmon resonance BaTiO3 BaTiO3 nanoparticles Composite photocatalysts Diffuse reflectance spectroscopy Modification Photo catalytic degradation Photocatalytic reduction Photogenerated electrons |
ISSN号 | 10053093 |
DOI | 10.11901/1005.3093.2016.222 |
英文摘要 | BaTiO3 nanoparticles were fabricated by gel method with polyacrylamide as raw material, and then Au nanoparticles were deposited on the surface of BaTiO3 via a photocatalytic reduction method to yield Au/BaTiO3 composite photocatalysts. The composite photocatalysts were characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), ultraviolet-visible diffuse reflectance spectroscopy (UV-Vis DRS) and photoluminescence (PL) spectroscopy. The results show that the BaTiO3 particles undergo no structural change after the deposition of gold; The Au particles with size of 5-20 nm were deposited on the surface of BaTiO3 particles with an average size of ~55 nm; The composites present light absorbance centered around 560 nm due to the surface plasmon resonance (SPR) effect of Au nanoparticles; The Au/BaTiO3 composites exhibit a reduction in recombination probability of photo-generated electrons and holes compared to bare BaTiO3. In addition, the formation mechanism for Au nanoparticles on the surface of BaTiO3 particles is proposed. The photocatalytic activity of the as-prepared composite photocatalyst was evaluated by the degradation of methylene blue (MB) under simulated sunlight irradiation, and the photocatalytic stability of the composites was also investigated. The results reveal that the photocatalytic activity of BaTiO3 can be improved by the deposition of appropriate amount of gold, and moreover the composite photocatalyst exhibits good reusability. Finally, the promotion mechanism of Au particles on the simulated sunlight photocatalytic activity of BaTiO3 is also discussed. © All right reserved. |
语种 | 中文 |
出版者 | Chinese Journal of Materials Research |
内容类型 | 期刊论文 |
源URL | [http://ir.lut.edu.cn/handle/2XXMBERH/114679] |
专题 | 兰州理工大学 |
作者单位 | 1.Department of Physics, Qinghai Normal University, Xining; 810008, China; 2.State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals, Lanzhou University of Technology, Lanzhou; 730050, China |
推荐引用方式 GB/T 7714 | Xian, Tao,Di, Lijing,Ma, Jun,et al. Photocatalytic degradation activity of BaTiO3 nanoparticles modified with au in simulated sunlight[J]. Cailiao Yanjiu Xuebao/Chinese Journal of Materials Research,2017,31(2):102-109. |
APA | Xian, Tao,Di, Lijing,Ma, Jun,Sang, Cuicui,Wei, Xuegang,&Zhou, Yongjie.(2017).Photocatalytic degradation activity of BaTiO3 nanoparticles modified with au in simulated sunlight.Cailiao Yanjiu Xuebao/Chinese Journal of Materials Research,31(2),102-109. |
MLA | Xian, Tao,et al."Photocatalytic degradation activity of BaTiO3 nanoparticles modified with au in simulated sunlight".Cailiao Yanjiu Xuebao/Chinese Journal of Materials Research 31.2(2017):102-109. |
个性服务 |
查看访问统计 |
相关权益政策 |
暂无数据 |
收藏/分享 |
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。
修改评论