One-step fabrication of Fe3O4-Cu nanocomposites: High-efficiency and low-cost catalysts for reduction of 4-nitrophenol
W. S. Zhao; S. Yang; C. Z. Guo; J. H. Yang and Y. Liu
刊名Materials Chemistry and Physics
2021
卷号260页码:5
ISSN号0254-0584
DOI10.1016/j.matchemphys.2020.124144
英文摘要Transition metal Cu nanocrystals have shown promising prospects for degrading organic pollutants. Herein, high efficiency Fe3O4-Cu nanocomposites (NCs) have been successfully synthesized though a facile one-step thermal decomposition method. With a turnover frequency of 6.4 min(-1), our Fe3O4-Cu NCs (heated temperature: 225 degrees C) could degrade the 4-nitrophenol in less than 15 s and showed almost unchanged catalytic efficiency (>90%) after recycled reactions up to six times. Furthermore, the influence of the heat treatment on the structure, elemental distribution, magnetic property and catalytic performance of Fe3O4-Cu NCs was investigated. As the temperature increased from 225 degrees C to 285 degrees C, the saturation magnetization of Fe3O4-Cu NCs decreased from 7.27 to 26.2 emu/g, owing to the enlarged mass ratio of Fe3O4 nanocrystals: Cu nanocrystals. This work provides the practical design guidance to the large-scale fabrication of high-efficiency and low-cost Fe3O4-Cu NCs catalysts, which shows promising future for degrading the nitro compounds in wastewater.
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内容类型期刊论文
源URL[http://ir.ciomp.ac.cn/handle/181722/65483]  
专题中国科学院长春光学精密机械与物理研究所
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W. S. Zhao,S. Yang,C. Z. Guo,et al. One-step fabrication of Fe3O4-Cu nanocomposites: High-efficiency and low-cost catalysts for reduction of 4-nitrophenol[J]. Materials Chemistry and Physics,2021,260:5.
APA W. S. Zhao,S. Yang,C. Z. Guo,&J. H. Yang and Y. Liu.(2021).One-step fabrication of Fe3O4-Cu nanocomposites: High-efficiency and low-cost catalysts for reduction of 4-nitrophenol.Materials Chemistry and Physics,260,5.
MLA W. S. Zhao,et al."One-step fabrication of Fe3O4-Cu nanocomposites: High-efficiency and low-cost catalysts for reduction of 4-nitrophenol".Materials Chemistry and Physics 260(2021):5.
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