Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology

doi:10.1021/acsami.0c14551

	Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology
	Jiao, Shouzheng 4; Sun, Zhicheng 4; Wen, Jinyue 4; Liu, Yuanyuan 1; Li, Furong 4; Miao, Qingqing 2,3; Wu, Weixia 4; Li, Luhai 4; Zhou, Yang 1
刊名	ACS APPLIED MATERIALS & INTERFACES
	2020-10-28
卷号	12 期号:43 页码:48794-48803
关键词	dye-sensitized solar cells SiO2 aerogel quasi-solid-state electrolyte rapid curing screen printing
ISSN号	1944-8244
DOI	10.1021/acsami.0c14551
英文摘要	Gratzel's dye-sensitized solar cells (DSSCs) can readily convert sunlight into electricity, attracting considerable attention of global scientists. The fabrication efficiency of DSSCs was greatly limited by the slow fabrication (similar to 3.5-24 h) of quasi-solid (QS) electrolytes to date. In this study, novel composites of SiO2 aerogel with graphene (GR), multi-walled carbon nanotubes, or polyaniline were proposed in the fabrication of QS-state electrolytes. The morphology of these composites was characterized. The gels with SiO2 aerogels as QS electrolytes of DSSCs can be rapidly cured in similar to 3 s. Using the screen-printing technology, these QS electrolytes can be readily utilized to construct the QS-DSSC to provide high efficiency and great stability. The photovoltaic parameters and interfacial chargetransfer resistances of the QS-DSSC incorporated with our synthetic composites were investigated in detail. Specifically, the SiO2 aerogel composed of GR (SiO2@GR) as a gel can greatly improve the performance of QS-DSSCs up to 8.25%. It is likely that these SiO2 aerogel composite electrolytes could provide a rapid curing process in the preparation of QS-state DSSCs, which might be useful to promote the development of DSSCs for future industrialization.
资助项目	National Natural Science Foundation of China[21776021] ; National Natural Science Foundation of China[21646013] ; National Natural Science Foundation of China[22007025] ; National Natural Science Foundation of China[21878309] ; National Natural Science Foundation of China[22078340] ; Key Scientific Research Project of Beijing Municipal commission of Education[KZ201910015016] ; BIGC Project[Ec202004] ; Youth Innovation Promotion Association, Chinese Academy of Sciences (CAS) ; Natural Science Foundation of Hebei Province[E2019103008] ; Hainan University[KYQD (ZR)20041] ; Hainan University[KYQD (ZR) 20040]
WOS关键词	GEL POLYMER ELECTROLYTES ; SILICA NANOPARTICLES ; IONIC LIQUID ; HIGH-EFFICIENCY ; PHOTOVOLTAIC PERFORMANCE ; REDOX ELECTROLYTE ; HOLE TRANSFER ; SURFACE-AREA ; LOW-COST ; HYBRID
WOS研究方向	Science & Technology - Other Topics ; Materials Science
语种	英语
出版者	AMER CHEMICAL SOC
WOS记录号	WOS:000586868400056
资助机构	National Natural Science Foundation of China ; Key Scientific Research Project of Beijing Municipal commission of Education ; BIGC Project ; Youth Innovation Promotion Association, Chinese Academy of Sciences (CAS) ; Natural Science Foundation of Hebei Province ; Hainan University
内容类型	期刊论文
源URL	[http://ir.ipe.ac.cn/handle/122111/42686]
专题	中国科学院过程工程研究所
通讯作者	Sun, Zhicheng; Miao, Qingqing; Zhou, Yang
作者单位	1.Hainan Univ, Sch Chem Engn & Technol, Minist Educ, Key Lab Adv Mat Trop Isl Resources, Haikou 570228, Hainan, Peoples R China 2.Chinese Acad Sci, Langfang Inst Proc Engn, Langfang 065001, Peoples R China 3.Chinese Acad Sci, Inst Proc Engn, CAS Key Lab Green Proc & Engn, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China 4.Beijing Inst Graph Commun, Beijing Engn Res Ctr Printed Elect, Beijing 102600, Peoples R China
推荐引用方式 GB/T 7714	Jiao, Shouzheng,Sun, Zhicheng,Wen, Jinyue,et al. Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology[J]. ACS APPLIED MATERIALS & INTERFACES,2020,12(43):48794-48803.
APA	Jiao, Shouzheng.,Sun, Zhicheng.,Wen, Jinyue.,Liu, Yuanyuan.,Li, Furong.,...&Zhou, Yang.(2020).Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology.ACS APPLIED MATERIALS & INTERFACES,12(43),48794-48803.
MLA	Jiao, Shouzheng,et al."Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology".ACS APPLIED MATERIALS & INTERFACES 12.43(2020):48794-48803.