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Enhanced treatment performance of phenol wastewater by electrochemical reactor with MnOx/Ti membrane electrode modified with Sb-SnO(2)interlayer People's Republic of China
Fan, Xiaowei1,2; Liang, Xiaoping2; Zhao, Zenghua3; Zhang, Di2; Liu, Hongying2; Zhang, Yuanyang2; Wang, Hong2; Li, Jianxin2
刊名JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
2020-09-23
页码12
ISSN号0957-4522
DOI10.1007/s10854-020-04441-0
英文摘要Sb-SnO2/Ti electrode membrane was prepared by loading Sb-SnO(2)polymer precursor on the original Ti substrate electrode membrane, then MnO(x)sol was coated on the surface of Sb-SnO2/Ti to obtain MnOx/Sb-SnO2/Ti composite electrode membrane via sol-gel method. Compared with MnOx/Ti, the new crystal form and solid solution were identified in MnOx/Sb-SnO2/Ti due to the presence of Sb-SnO(2)interlayer, which was beneficial to improve the electrochemical performance of MnOx/Ti. In particular, the specific surface area of MnOx/Ti was increased by inserting Sb-SnO(2)interlayer. Electrocatalytic membrane reactor (ECMR) is assembled with the electrode membrane as the anode and the stainless-steel mesh as the cathode for phenolic wastewater treatment. pH value and Sb-SnO2-loading amount had great effect on the energy consumption of ECMR. When the current density, residence time and Sb-SnO(2)loading were 0.9 mA/cm(2), 15 min and 3.4 wt%, the phenol and COD degradation rate of ECMR with MnOx/Sb-SnO2/Ti reached 98.98% and 89.38%, whereas were 80.56% and 71.12% in case of MnOx/Ti, respectively.
资助项目National Natural Science Foundation of China[21878230] ; National Natural Science Foundation of China[21576208] ; Science and Technology Planning Projects of Tianjin[17JCYBJC18PTZWH Z00210] ; Program for Innovative Research Team in University of Ministry of Education of China[IRT17R80]
WOS关键词ELECTROCATALYTIC OXIDATION ; CONTROLLABLE OXIDATION ; OXIDE ; REMOVAL ; FENTON ; FILMS ; ACID
WOS研究方向Engineering ; Materials Science ; Physics
语种英语
出版者SPRINGER
WOS记录号WOS:000572323900010
资助机构National Natural Science Foundation of China ; Science and Technology Planning Projects of Tianjin ; Program for Innovative Research Team in University of Ministry of Education of China
内容类型期刊论文
源URL[http://ir.ipe.ac.cn/handle/122111/42221]  
专题中国科学院过程工程研究所
通讯作者Liang, Xiaoping; Li, Jianxin
作者单位1.Tianjin SYP Engn Glass Co Ltd, Tianjin 300409, Peoples R China
2.Tianjin Polytech Univ, State Key Lab Separat Membranes & Membrane Proc, Natl Ctr Int Joint Res Separat Membranes, Sch Mat Sci & Engn, Tianjin 300387, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Fan, Xiaowei,Liang, Xiaoping,Zhao, Zenghua,et al. Enhanced treatment performance of phenol wastewater by electrochemical reactor with MnOx/Ti membrane electrode modified with Sb-SnO(2)interlayer People's Republic of China[J]. JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,2020:12.
APA Fan, Xiaowei.,Liang, Xiaoping.,Zhao, Zenghua.,Zhang, Di.,Liu, Hongying.,...&Li, Jianxin.(2020).Enhanced treatment performance of phenol wastewater by electrochemical reactor with MnOx/Ti membrane electrode modified with Sb-SnO(2)interlayer People's Republic of China.JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS,12.
MLA Fan, Xiaowei,et al."Enhanced treatment performance of phenol wastewater by electrochemical reactor with MnOx/Ti membrane electrode modified with Sb-SnO(2)interlayer People's Republic of China".JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS (2020):12.
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