Improved antibiofouling properties of photobioreactor with amphiphilic sulfobetaine copolymer coatings | |
Wang, Yixuan1,2; Chen, Caixiang1,2; Wu, Xia2; Wang, Zhihui2; Wen, Shumei2; Yu, Jing2; Yan, Chenghu2; Cong, Wei2 | |
刊名 | PROGRESS IN ORGANIC COATINGS
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2020-07-01 | |
卷号 | 144页码:7 |
关键词 | Biofouling Photobioreactor Microlagae cultivation Sulfobetaine Amphiphilic copolymers |
ISSN号 | 0300-9440 |
DOI | 10.1016/j.porgcoat.2020.105666 |
英文摘要 | Biofouling is a critical challenge for the commercial application of photobioreactors for microalgae cultivation. In this work, a series of amphiphilic sulfobetaine copolymers (ASC) with different ratios of sulfobetaine (SBMA) and 2, 2, 2-trifluoroethyl methacrylate (TFMA) were synthesized via a monomer-starved seeded semi-continous emulsion polymerization method and were used to improve the antibiofouling capability of ethylene-vinyl acetate copolymer (EVA) film by surface coating method. Effects of the SBMA/TFMA ratio on the resultant ASC latexes and coating properties were investigated. With the increase of the SBMA/TFMA ratio, the particle diameter, polydispersity index and water uptake of ASC latexes and coating decreased from 261.8 nm to 144.9 nm, 0.198 to 0.054 and 26.28 % to 7.84 %, respectively, and increased afterwards. Fourier transform Infrared (FT-IR) spectra and X-ray photoelectron spectroscopy analysis (XPS) indicated that SBMA and TFMA were introduced onto the EVA film surface successfully. The contact angle of ASC modified EVA (EVA-ASC) film sharply decreased after immersed in water. The EVA-ASC film either in dry, or in water swollen state exhibited excellent optical transparency in the visible light. The adsorption of bovine serum albumin and Chlorella sp. on the EVA-ASC surface was investigated with protein and microalgae adsorption assay. It was shown that the EVA-ASC film had excellent protein and microalgae absorption resisting characteristic, the density of absorbed protein and microalgae decreased 92 % and 50 % compared with those of EVA film, respectively. |
资助项目 | Natural Science Foundation of China[21706260] ; National key R&D Program of China[2016YFC0500904] |
WOS关键词 | ZWITTERIONIC POLYMER ; FOULING RESISTANCE ; SURFACES ; TRITHIOCARBONATE ; DESIGN |
WOS研究方向 | Chemistry ; Materials Science |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE SA |
WOS记录号 | WOS:000557819500010 |
资助机构 | Natural Science Foundation of China ; National key R&D Program of China |
内容类型 | 期刊论文 |
源URL | [http://ir.ipe.ac.cn/handle/122111/41679] ![]() |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Yan, Chenghu; Cong, Wei |
作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Yixuan,Chen, Caixiang,Wu, Xia,et al. Improved antibiofouling properties of photobioreactor with amphiphilic sulfobetaine copolymer coatings[J]. PROGRESS IN ORGANIC COATINGS,2020,144:7. |
APA | Wang, Yixuan.,Chen, Caixiang.,Wu, Xia.,Wang, Zhihui.,Wen, Shumei.,...&Cong, Wei.(2020).Improved antibiofouling properties of photobioreactor with amphiphilic sulfobetaine copolymer coatings.PROGRESS IN ORGANIC COATINGS,144,7. |
MLA | Wang, Yixuan,et al."Improved antibiofouling properties of photobioreactor with amphiphilic sulfobetaine copolymer coatings".PROGRESS IN ORGANIC COATINGS 144(2020):7. |
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