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A facile strategy to form three-dimensional network structure for mechanically robust superhydrophobic nanocoatings with enhanced transmittance
Xi, Rubing1; Wang, Yabin2; Li, Xiaoyu3; Zhang, Xueji1; Du, Xin1
刊名JOURNAL OF COLLOID AND INTERFACE SCIENCE
2020-03-15
卷号563页码:42-53
关键词Antireflective Nanocoatings Superhydrophobic Self-cleaning Mechanical Robustness Three-dimensional Network Structure Balanced Properties
ISSN号0021-9797
DOI10.1016/j.jcis.2019.12.049
英文摘要

The mechanically robust nanocoatings with high transmittance and superhydrophobic self-cleaning are widely desired in daily-life and industry. However, to the state-of-art, it is still a great challenge to develop a simple and cost-effective approach to construct a multifunctional nanocoating due to structural confliction and technical limitation. In this work, we successfully fabricated such a multifunctional nanocoating through dip-coating a mixed suspension composed of acid-catalyzed silica sol (ACSS) as binder and hydrophobic silica nanoparticles (HSNs) as building block onto the glass substrate without any post-treatments. The introduction of ACSS highly crosslinked the HSNs and formed three-dimensional network structure, which enhanced the adhesion between HSNs and substrate, and thus significantly improved mechanical robustness of the nanocoatings. Moreover, it also retained enough porosity and surface roughness, thus achieving high transmittance and superhydrophobicity. The optimized nanocoating deposited on the glass slide had high transmittance of 96.17% and superhydrophobic self-cleaning property. It also showed highly mechanical robustness (3H pencil scratching test), enhanced adhesion (class of 4B for tape adhesion test), weatherable, and acidic (pH 5.0)/alkaline (pH 10.0) and thermal (250 degrees C) stability. The multifunctional nanocoating with the comprehensive performance has great potentials in practical applications. (C) 2019 Elsevier Inc. All rights reserved.

资助项目Fundamental Research Funds for the Central Universities[230201506500017] ; Fundamental Research Funds for the Central Universities[FRF-BR-17-032A] ; Fundamental Research Funds for the Central Universities[FRF-BR-17-002B] ; Fundamental Research Funds for the Central Universities[FRF-BD-17-016A] ; National Natural Science Foundation of China[21501009] ; National Natural Science Foundation of China[51671181] ; Natural Science Basic Research Plan in Shaanxi Province of China[2019JQ-104] ; Beijing Municipal Science and Technology Commission[z131102002813058]
WOS关键词Antireflective Coatings ; Silica Nanoparticles ; High-performance ; Transparent ; Surfaces ; Fabrication ; Nanospheres ; Resistant ; Films
WOS研究方向Chemistry
语种英语
出版者ACADEMIC PRESS INC ELSEVIER SCIENCE
WOS记录号WOS:000510313700006
资助机构Fundamental Research Funds for the Central Universities ; National Natural Science Foundation of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; Beijing Municipal Science and Technology Commission
内容类型期刊论文
源URL[http://ir.ipe.ac.cn/handle/122111/39282]  
专题中国科学院过程工程研究所
通讯作者Wang, Yabin
作者单位1.Univ Sci & Technol Beijing, Res Ctr Bioengn & Sensing Technol, Dept Chem & Biol Engn, Beijing 100083, Peoples R China
2.Yanan Univ, Coll Chem & Chem Engn, Shaanxi Key Lab Chem React Engn, Yanan 716000, Shaanxi, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Xi, Rubing,Wang, Yabin,Li, Xiaoyu,et al. A facile strategy to form three-dimensional network structure for mechanically robust superhydrophobic nanocoatings with enhanced transmittance[J]. JOURNAL OF COLLOID AND INTERFACE SCIENCE,2020,563:42-53.
APA Xi, Rubing,Wang, Yabin,Li, Xiaoyu,Zhang, Xueji,&Du, Xin.(2020).A facile strategy to form three-dimensional network structure for mechanically robust superhydrophobic nanocoatings with enhanced transmittance.JOURNAL OF COLLOID AND INTERFACE SCIENCE,563,42-53.
MLA Xi, Rubing,et al."A facile strategy to form three-dimensional network structure for mechanically robust superhydrophobic nanocoatings with enhanced transmittance".JOURNAL OF COLLOID AND INTERFACE SCIENCE 563(2020):42-53.
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