Robust superhydrophobic fabric via UV-accelerated atmospheric deposition of polydopamine and silver nanoparticles for solar evaporation and water/oil separation | |
Zhang, Hongliang2; Ou, Junfei2; Fang, Xinzuo2; Lei, Sheng2; Wang, Fajun2; Li, Changquan2; Li, Wen2; Hu, Yating1,2; Amirfazli, Alidad1; Wang, Peng3 | |
刊名 | CHEMICAL ENGINEERING JOURNAL |
2022-02-01 | |
卷号 | 429页码:14 |
关键词 | Lotus effect Mussel effect Bio-inspired Desalination Membrane |
ISSN号 | 1385-8947 |
DOI | 10.1016/j.cej.2021.132539 |
通讯作者 | Ou, Junfei(oujunfei_1982@163.com) ; Wang, Peng(wangpeng@qdio.ac.cn) |
英文摘要 | Polydopamine (PDA) inspired by mussel plays a unique role in surface modification due to its strong adhesion to virtually all kinds of materials and the subsequent functionality. However, the deposition of PDA and its subsequent metallization in bulk solution is slow and thus the surface modification based on PDA is not efficient. Herein, by atmospheric deposition with the aid of ultraviolet (UV) irradiation, a process is proposed to facilitate the fast deposition of PDA and silver nanpparticles (Ag NPs) on cotton fabric. The word "fast" means that efficiency of the overall deposition is increased by 45 times. Fabric with PDA and Ag NPs is further modified by dodecyl mercaptan (DT) and turns to be superhydrophobic. Ag NPs play multiple roles in the fabrication and application of the superhydrophobic fabric, viz., enhancing the hydrophobicity and photothermal effect of the fabric. Due to its superhydrophobicity and excellent photothermal effect, the fabric floating on water can harvest solar energy to facilitate the local evaporation of seawater. The evaporation rate is 1.66 kg/(m(2).h) and the solar energy conversion efficiency is 91%. As the oil-water separation membrane, the separation efficiency of oil-water mixture is more than 96%, and the oil flux is more than 12 m(3).m(-2).h(-1). Overall, this is a story from sea to sea. PDA inspired by the sea creature of mussel is quickly deposited on the fabric and serves as a platform for further deposition of silver and modification with DT, and the so-obtained superhydrophobic sample can be used to solve the marine problems such as solar evaporation and oil/water separation. |
资助项目 | National Natural Science Foundation of China[52073127] ; National Natural Science Foundation of China[41922040] ; Changzhou Sci Tech Program[CM20193004] ; Natural Science Foundation of Jiangsu Province[BK20211359] |
WOS研究方向 | Engineering |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE SA |
WOS记录号 | WOS:000728573800006 |
内容类型 | 期刊论文 |
源URL | [http://ir.qdio.ac.cn/handle/337002/177494] |
专题 | 海洋研究所_海洋腐蚀与防护研究发展中心 |
通讯作者 | Ou, Junfei; Wang, Peng |
作者单位 | 1.York Univ, Dept Mech Engn, Toronto, ON M3J 1P3, Canada 2.Jiangsu Univ Technol, Sch Mat Engn, Changzhou 213001, Peoples R China 3.Chinese Acad Sci, Inst Oceanol, Key Lab Marine Environm Corros & Biofouling, 7 Nanhai Rd, Qingdao 266071, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Hongliang,Ou, Junfei,Fang, Xinzuo,et al. Robust superhydrophobic fabric via UV-accelerated atmospheric deposition of polydopamine and silver nanoparticles for solar evaporation and water/oil separation[J]. CHEMICAL ENGINEERING JOURNAL,2022,429:14. |
APA | Zhang, Hongliang.,Ou, Junfei.,Fang, Xinzuo.,Lei, Sheng.,Wang, Fajun.,...&Wang, Peng.(2022).Robust superhydrophobic fabric via UV-accelerated atmospheric deposition of polydopamine and silver nanoparticles for solar evaporation and water/oil separation.CHEMICAL ENGINEERING JOURNAL,429,14. |
MLA | Zhang, Hongliang,et al."Robust superhydrophobic fabric via UV-accelerated atmospheric deposition of polydopamine and silver nanoparticles for solar evaporation and water/oil separation".CHEMICAL ENGINEERING JOURNAL 429(2022):14. |
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