Probing the Influence of the Substrate Hole Shape on the Interaction between Helium Ions and Suspended Monolayer Graphene with Raman Spectroscopy
He, Shixuan2,3; Xie, Wanyi1,2; Zhang, Yongna2; Fang, Shaoxi1,2; Zhou, Daming2; Gan, Jie2; Zhang, Zhiyou3; Du, Jinglei3; Du, Chunlei3; Wang, Deqiang1,2
刊名JOURNAL OF PHYSICAL CHEMISTRY C
2021-01-28
卷号125期号:3页码:2202-2211
ISSN号1932-7447
DOI10.1021/acs.jpcc.0c10738
通讯作者Du, Chunlei(mscldu@cigit.ac.cn) ; Wang, Deqiang(dqwang@cigit.ac.cn)
英文摘要A helium ion beam (HIB) is ideal for milling monolayer graphene in nanopore applications, but the optimizing irradiation parameter requires a comprehensive microscopic understanding of the interaction between helium ions and the suspended graphene. In this work, we investigate the influence of the substrate hole shape on the interaction between helium ions and suspended monolayer graphene on a substrate with periodic structures of different shapes. Raman spectroscopy is used to correlate the dose of HIB irradiation with engineered defects on freestanding monolayer graphene. Raman characteristics of the suspended monolayer graphene are related to the pore size and shape of the supporting substrate upon helium ion irradiation. These provide insights into the influence of the substrate hole shape on the interaction between helium ions and a freestanding graphene membrane. Our results can be used to analyze ion-membrane interactions in the other suspended monolayer two-dimensional materials for sub-nanometer precision nanopore fabrication.
资助项目Youth Innovation Foundation of CIGIT ; Natural Science Foundation of Chongqing, China[cstc2018jcyjAX0310] ; Natural Science Foundation of Chongqing, China[cstc2018jcyjAX0308] ; Instrument development program of CAS[YZ201568]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000614317500058
内容类型期刊论文
源URL[http://119.78.100.138/handle/2HOD01W0/13029]  
专题中国科学院重庆绿色智能技术研究院
通讯作者Du, Chunlei; Wang, Deqiang
作者单位1.Univ Chinese Acad Sci, Chongqing Sch, Chongqing 400714, Peoples R China
2.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
3.Sichuan Univ, Coll Phys, Chengdu 610065, Sichuan, Peoples R China
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He, Shixuan,Xie, Wanyi,Zhang, Yongna,et al. Probing the Influence of the Substrate Hole Shape on the Interaction between Helium Ions and Suspended Monolayer Graphene with Raman Spectroscopy[J]. JOURNAL OF PHYSICAL CHEMISTRY C,2021,125(3):2202-2211.
APA He, Shixuan.,Xie, Wanyi.,Zhang, Yongna.,Fang, Shaoxi.,Zhou, Daming.,...&Wang, Deqiang.(2021).Probing the Influence of the Substrate Hole Shape on the Interaction between Helium Ions and Suspended Monolayer Graphene with Raman Spectroscopy.JOURNAL OF PHYSICAL CHEMISTRY C,125(3),2202-2211.
MLA He, Shixuan,et al."Probing the Influence of the Substrate Hole Shape on the Interaction between Helium Ions and Suspended Monolayer Graphene with Raman Spectroscopy".JOURNAL OF PHYSICAL CHEMISTRY C 125.3(2021):2202-2211.
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