Distribution and vertical migration of polycyclic aromatic hydrocarbons in forest soil pits of southeastern Tibet
Xue, Yonggang1,2,3; Wang, Xiaoping2,3; Gong, Ping2,3; Yao, Tandong2,3
刊名ENVIRONMENTAL GEOCHEMISTRY AND HEALTH
2018-10-01
卷号40期号:5页码:1941-1953
关键词PAHs Forest soil Southeastern Tibet Vertical migration
ISSN号0269-4042
DOI10.1007/s10653-017-9969-7
通讯作者Wang, Xiaoping(wangxp@itpcas.ac.cn)
英文摘要PAHs could be transported to Tibetan Plateau in accompany with atmospheric circulation. The forest regions were found be an important sink for PAHs, while their distributions and migrations in forest are still uncertain. In this study, soil profile samples were collected in southeastern Tibet and the concentrations, distributions, and migration of PAHs in forest region were investigated. The PAHs levels in the forest soils were at the low end of remote sites, ranged from 27.4 to 120.3 ng g(-1) on a dry weight based. Due to low ambient temperature and high organic carbon content, enrichment of PAHs was found in higher altitude on north side. According to the soil profiles, the vertical distributions of PAHs in organic layers were mainly influenced by pedogenesis, while the vertical distributions in mineral layers were dominated by downward leaching effect. Enrich factor (EF) of PAHs was estimated, and the values in organic layers were positively correlated with the octanol-air partition coefficients (K-OA), but EFs in mineral layers decreased with the K-OA values. PAHs in the surface soils on the north side of forest were relatively stable, while the migration of PAHs on the south sides and other clearing sites was more active. The leaching rates of PAHs in clearing site ranged between 1.42 and 29.3%. The results from this study are valuable on the characterization of PAHs in Tibetan Plateau.
资助项目National Natural Science Foundation of China[41071321] ; National Natural Science Foundation of China[41671480] ; Youth Innovation Promotion Association[CAS2011067]
WOS关键词PERSISTENT ORGANIC POLLUTANTS ; POLYCHLORINATED-BIPHENYLS ; ORGANOCHLORINE PESTICIDES ; SOURCE APPORTIONMENT ; ATMOSPHERIC DEPOSITION ; SPATIAL-DISTRIBUTION ; WESTERN SICHUAN ; SURFACE SOIL ; BLACK CARBON ; PAHS
WOS研究方向Engineering ; Environmental Sciences & Ecology ; Public, Environmental & Occupational Health ; Water Resources
语种英语
出版者SPRINGER
WOS记录号WOS:000452158700019
资助机构National Natural Science Foundation of China ; Youth Innovation Promotion Association
内容类型期刊论文
源URL[http://ir.ieecas.cn/handle/361006/14492]  
专题地球环境研究所_黄土与第四纪地质国家重点实验室(2010~)
通讯作者Wang, Xiaoping
作者单位1.Chinese Acad Sci, Key Lab Aerosol Chem & Phys, SKLLQG, Inst Earth Environm, Xian 710061, Peoples R China
2.CAS Ctr Excellence Tibetan Plateau Earth Sci, Beijing 100101, Peoples R China
3.Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing 100101, Peoples R China
推荐引用方式
GB/T 7714
Xue, Yonggang,Wang, Xiaoping,Gong, Ping,et al. Distribution and vertical migration of polycyclic aromatic hydrocarbons in forest soil pits of southeastern Tibet[J]. ENVIRONMENTAL GEOCHEMISTRY AND HEALTH,2018,40(5):1941-1953.
APA Xue, Yonggang,Wang, Xiaoping,Gong, Ping,&Yao, Tandong.(2018).Distribution and vertical migration of polycyclic aromatic hydrocarbons in forest soil pits of southeastern Tibet.ENVIRONMENTAL GEOCHEMISTRY AND HEALTH,40(5),1941-1953.
MLA Xue, Yonggang,et al."Distribution and vertical migration of polycyclic aromatic hydrocarbons in forest soil pits of southeastern Tibet".ENVIRONMENTAL GEOCHEMISTRY AND HEALTH 40.5(2018):1941-1953.
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