The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China | |
Wang, Xudong1,2,3; Liu, Guijian2,3; Zhou, Chuncai2,3 | |
刊名 | ENVIRONMENTAL FORENSICS
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2019-08-28 | |
页码 | 10 |
关键词 | Coal combustion trace elements partition behavior environmental impacts |
ISSN号 | 1527-5922 |
DOI | 10.1080/15275922.2019.1657984 |
通讯作者 | Liu, Guijian(lgj@ustc.edu.cn) |
英文摘要 | The trace elements (TEs) in coal are of great concern due to their toxicity and bioavailability. The coal, bottom ash, fly ash and gaseous species were sampled to study the partitioning and environmental behaviors of TEs during coal combustion. The mineral and phase characterizations of coal combustion residue were determined by X-ray powder diffraction (XRD) and fourier transform infrared spectroscopy (FTIR), respectively. The gaseous emission, risk assessment code and leaching experiment EN 12457 Part 2 procedure were employed to assess the potential environmental impacts. The concentrations of TEs in all the collected samples were determined by inductively coupled plasma mass spectrometry (ICP-MS). During combustion, the mineral compositions of coal (kaolinite, quartz, illite, pyrite and calcite) were changed to mullite, quartz, hematite, lime, magnetite and anhydrite. Arsenic, Cd, Cu, Pb and Zn were emitted mainly in fly ash and gaseous phases. In the current unconfined deposits, the TEs (As, Cu, Pb and Zn) in bottom ash and fly ash may pose a medium risk to the environment. High regularization and management countermeasures including immobilization/stabilization, re-utilization of combustion ash, and controlled disposal should be conducted to eliminate/minimize environmental and ecological risks in coal activities areas. |
资助项目 | National Basic Research Program of China (973 Program)[2016YFC0201600] ; National Natural Science Foundation of China[41702166] ; National Natural Science Foundation of China[41672144] ; Anhui Provincial Natural Science Foundation[1708085QE110] ; National Postdoctoral Program for Innovative Talents[BX201700222] ; China Postdoctoral Science Foundation[2017M622011] |
WOS关键词 | CHEMICAL-COMPOSITION ; FLY ASHES ; MULTICOMPONENT UTILIZATION ; FEED COALS ; COMBUSTION ; FATE ; METALS ; MATTER ; VOLATILITY ; MINERALOGY |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | TAYLOR & FRANCIS LTD |
WOS记录号 | WOS:000484135700001 |
资助机构 | National Basic Research Program of China (973 Program) ; National Natural Science Foundation of China ; Anhui Provincial Natural Science Foundation ; National Postdoctoral Program for Innovative Talents ; China Postdoctoral Science Foundation |
内容类型 | 期刊论文 |
源URL | [http://ir.ieecas.cn/handle/361006/13512] ![]() |
专题 | 地球环境研究所_黄土与第四纪地质国家重点实验室(2010~) |
通讯作者 | Liu, Guijian |
作者单位 | 1.Anhui Publ Welf Geol Survey Management Ctr, Dept Nat Resources Anhui Prov, Hefei, Anhui, Peoples R China 2.Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China 3.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Shaanxi, Peoples R China |
推荐引用方式 GB/T 7714 | Wang, Xudong,Liu, Guijian,Zhou, Chuncai. The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China[J]. ENVIRONMENTAL FORENSICS,2019:10. |
APA | Wang, Xudong,Liu, Guijian,&Zhou, Chuncai.(2019).The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China.ENVIRONMENTAL FORENSICS,10. |
MLA | Wang, Xudong,et al."The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China".ENVIRONMENTAL FORENSICS (2019):10. |
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