The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China
Wang, Xudong1,2,3; Liu, Guijian2,3; Zhou, Chuncai2,3
刊名ENVIRONMENTAL FORENSICS
2019-08-28
页码10
关键词Coal combustion trace elements partition behavior environmental impacts
ISSN号1527-5922
DOI10.1080/15275922.2019.1657984
通讯作者Liu, Guijian(lgj@ustc.edu.cn)
英文摘要The trace elements (TEs) in coal are of great concern due to their toxicity and bioavailability. The coal, bottom ash, fly ash and gaseous species were sampled to study the partitioning and environmental behaviors of TEs during coal combustion. The mineral and phase characterizations of coal combustion residue were determined by X-ray powder diffraction (XRD) and fourier transform infrared spectroscopy (FTIR), respectively. The gaseous emission, risk assessment code and leaching experiment EN 12457 Part 2 procedure were employed to assess the potential environmental impacts. The concentrations of TEs in all the collected samples were determined by inductively coupled plasma mass spectrometry (ICP-MS). During combustion, the mineral compositions of coal (kaolinite, quartz, illite, pyrite and calcite) were changed to mullite, quartz, hematite, lime, magnetite and anhydrite. Arsenic, Cd, Cu, Pb and Zn were emitted mainly in fly ash and gaseous phases. In the current unconfined deposits, the TEs (As, Cu, Pb and Zn) in bottom ash and fly ash may pose a medium risk to the environment. High regularization and management countermeasures including immobilization/stabilization, re-utilization of combustion ash, and controlled disposal should be conducted to eliminate/minimize environmental and ecological risks in coal activities areas.
资助项目National Basic Research Program of China (973 Program)[2016YFC0201600] ; National Natural Science Foundation of China[41702166] ; National Natural Science Foundation of China[41672144] ; Anhui Provincial Natural Science Foundation[1708085QE110] ; National Postdoctoral Program for Innovative Talents[BX201700222] ; China Postdoctoral Science Foundation[2017M622011]
WOS关键词CHEMICAL-COMPOSITION ; FLY ASHES ; MULTICOMPONENT UTILIZATION ; FEED COALS ; COMBUSTION ; FATE ; METALS ; MATTER ; VOLATILITY ; MINERALOGY
WOS研究方向Environmental Sciences & Ecology
语种英语
出版者TAYLOR & FRANCIS LTD
WOS记录号WOS:000484135700001
资助机构National Basic Research Program of China (973 Program) ; National Natural Science Foundation of China ; Anhui Provincial Natural Science Foundation ; National Postdoctoral Program for Innovative Talents ; China Postdoctoral Science Foundation
内容类型期刊论文
源URL[http://ir.ieecas.cn/handle/361006/13512]  
专题地球环境研究所_黄土与第四纪地质国家重点实验室(2010~)
通讯作者Liu, Guijian
作者单位1.Anhui Publ Welf Geol Survey Management Ctr, Dept Nat Resources Anhui Prov, Hefei, Anhui, Peoples R China
2.Univ Sci & Technol China, Sch Earth & Space Sci, CAS Key Lab Crust Mantle Mat & Environm, Hefei 230026, Anhui, Peoples R China
3.Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Shaanxi, Peoples R China
推荐引用方式
GB/T 7714
Wang, Xudong,Liu, Guijian,Zhou, Chuncai. The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China[J]. ENVIRONMENTAL FORENSICS,2019:10.
APA Wang, Xudong,Liu, Guijian,&Zhou, Chuncai.(2019).The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China.ENVIRONMENTAL FORENSICS,10.
MLA Wang, Xudong,et al."The partitioning and environmental characteristics of trace elements in a coal-fired power plant: a case study at Huaibei, China".ENVIRONMENTAL FORENSICS (2019):10.
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