Analysis of Iodine Isotopes in Travertine from Baishuitai, Yunnan Province, China
Zhang, Lu-Yuan2,3,4; Fang, Miao2,8; Sun, Hai-Long1; Hou, Xiao-Lin2,3,4; Cai, Yan-Jun5; Liu, Qi2; Chen, Ning2; Zhang, Tong2,6; Li, Tong2; Zhang, Zhi-Yong7
刊名ATOMIC SPECTROSCOPY
2020-09-01
卷号41期号:5页码:181-187
ISSN号0195-5373
DOI10.46770/AS.2020.05.001
通讯作者Zhang, Lu-Yuan(zhangly@ieecas.cn)
英文摘要Travertine and tufa can be used as a high-resolution record for reconstructing the paleoclimate and paleoenvironment. It is not clear whether travertine is able to preserve the radionuclides for the reconstruction of modern human nuclear events. In this study, we developed and compared two sample preparation methods for the determination of I-129 and I-127 in travertine samples using direct acid dissolution and pyrolysis combustion. The analytical results of the levels of I-129 and I-127 as well as the I-129/I-127 ratios in travertine are presented here for the first time, and the hydrodynamic influence on the levels and distribution of iodine isotopes are discussed. It was found that the concentration of I-127 in travertine was low in the winter but high in the summer. This temporal variation of I-127 is likely related to the level and species of iodine in the water supply by mixing geothermal water with rainfall, as well as the amount of iodine-containing impurity. The I-129 level clearly suggests that the Baishuitai travertine is endogenic and slightly affected by the amount of rainfall and biological impurities. The results of this study show that endogenic travertine can be used in reconstructing the influence of human nuclear activity with high resolution, and also imply that hypergenic tufa has great potential for such studies. Both archives have implications on the mechanism used for iodine incorporation into carbonate in the natural environment.
资助项目Youth Innovation Promotion Association of CAS[2019401] ; National Natural Science Foundation of China[11605207] ; National Natural Science Foundation of China[41603125] ; National Natural Science Foundation of China[41991252] ; Strategic Priority Research Program of Chinese Academy of Sciences[XDB40020104] ; Key Research Program of the Chinese Academy of Sciences[ZDRW-CN-2018-1]
WOS关键词CARRIER-FREE IODINE ; COPRECIPITATION SEPARATION ; NUCLEAR ACTIVITIES ; SW CHINA ; I-129 ; SAMPLES ; LEVEL ; I-129/I-127 ; AEROSOLS ; RATIOS
WOS研究方向Spectroscopy
语种英语
出版者ATOMIC SPECTROSCOPY PRESS LTD
WOS记录号WOS:000575494100001
资助机构Youth Innovation Promotion Association of CAS ; National Natural Science Foundation of China ; Strategic Priority Research Program of Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences
内容类型期刊论文
源URL[http://ir.ieecas.cn/handle/361006/15351]  
专题地球环境研究所_加速器质谱中心
第四纪科学与全球变化卓越创新中心
通讯作者Zhang, Lu-Yuan
作者单位1.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Peoples R China
2.Chinese Acad Sci, Xian AMS Ctr, Inst Earth Environm, State Key Lab Loess & Quaternary Geol,Shaanxi Key, Xian 710061, Peoples R China
3.Chinese Acad Sci, Ctr Excellence Quaternary Sci & Global Change, Xian 710061, Peoples R China
4.Pilot Natl Lab Marine Sci & Technol Qingdao, Open Studio Ocean Continental Climate & Environm, Qingdao 266061, Peoples R China
5.Xi An Jiao Tong Univ, Inst Global Environm Change, Xian 710061, Peoples R China
6.Xian Inst Innovat Earth Environm Res, Xian 710061, Peoples R China
7.Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China
8.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Lu-Yuan,Fang, Miao,Sun, Hai-Long,et al. Analysis of Iodine Isotopes in Travertine from Baishuitai, Yunnan Province, China[J]. ATOMIC SPECTROSCOPY,2020,41(5):181-187.
APA Zhang, Lu-Yuan.,Fang, Miao.,Sun, Hai-Long.,Hou, Xiao-Lin.,Cai, Yan-Jun.,...&Liu, Yi-Xuan.(2020).Analysis of Iodine Isotopes in Travertine from Baishuitai, Yunnan Province, China.ATOMIC SPECTROSCOPY,41(5),181-187.
MLA Zhang, Lu-Yuan,et al."Analysis of Iodine Isotopes in Travertine from Baishuitai, Yunnan Province, China".ATOMIC SPECTROSCOPY 41.5(2020):181-187.
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