Hierarchical mesoporous carbon nanosheets for efficient organic pollutants removal | |
Zheng, Yang; Niu, Hongyun; He, Dongwei; Wang, Saihua; Cai, Yaqi; Zhang, Shengxiao | |
刊名 | MICROPOROUS AND MESOPOROUS MATERIALS
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2019-03-01 | |
卷号 | 276页码:251-259 |
关键词 | Mesoporous carbon nanosheets 2,4,6-Trichlorophenol Adsorption |
ISSN号 | 1387-1811 |
英文摘要 | Hierarchical mesoporous carbon nanosheets were synthesized by using gallic acid and zinc organic-inorganic (Zn-GA) hybrids as templates. After carbonization and removal of ZnO nanoparticles by diluted HCl, carbon nanosheets with a thickness of 11-16 nm were formed and arranged like a completely-opened-erected book. The carbon nanosheets possessed mesopores (centered at 6.5 and 23.4 nm) and macropores and had high surface areas (786 m(2) g(-1)) and large pore volumes (1.57 cm(3) g(-1)). The thin thickness and high amount of mesopores of the carbon nanosheets ensured short diffusion path and largely available inner and outer adsorptive sites of the carbon nanosheet. The hierarchical structure of the carbon nanosheets avoided the thin nanosheets from aggregation during adsorption of organic pollutants in water solution. The obtained hierarchical mesoporous carbon (HMC) nanosheets were used as adsorbents to remove 2,4,6-trichlorophenol (TCP) from water. As a result, the HMC nanosheets showed fast adsorption rate and significantly higher adsorption capacity (833 mg g(-1)) to TCP than other mesoporous carbon materials. |
内容类型 | 期刊论文 |
源URL | [http://ir.rcees.ac.cn/handle/311016/42954] ![]() |
专题 | 生态环境研究中心_环境化学与生态毒理学国家重点实验室 |
作者单位 | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Ludong Univ, Sch Chem & Mat Sci, Yantai 264025, Peoples R China 4.Jianghan Univ, Inst Environm & Hlth, Wuhan 430056, Hubei, Peoples R China 5.Henan Chem Ind Res Inst Co Ltd, Zhengzhou 450052, Henan, Peoples R China |
推荐引用方式 GB/T 7714 | Zheng, Yang,Niu, Hongyun,He, Dongwei,et al. Hierarchical mesoporous carbon nanosheets for efficient organic pollutants removal[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2019,276:251-259. |
APA | Zheng, Yang,Niu, Hongyun,He, Dongwei,Wang, Saihua,Cai, Yaqi,&Zhang, Shengxiao.(2019).Hierarchical mesoporous carbon nanosheets for efficient organic pollutants removal.MICROPOROUS AND MESOPOROUS MATERIALS,276,251-259. |
MLA | Zheng, Yang,et al."Hierarchical mesoporous carbon nanosheets for efficient organic pollutants removal".MICROPOROUS AND MESOPOROUS MATERIALS 276(2019):251-259. |
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