Brominated flame retardants in atmospheric fine particles in the Beijing-Tianjin-Hebei region, China: Spatial and temporal distribution and human exposure assessment
Zhang, Weiwei; Wang, Pu; Zhu, Ying; Yang, Ruiqiang; Li, Yingming; Wang, Dou; Matsiko, Julius; Han, Xu; Zhao, Junpeng; Zhang, Qinghua
刊名ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY
2019-04-30
卷号171页码:181-189
关键词Novel brominated flame retardants Atmospheric fine particles The Beijing-Tianjin-Hebei region Spatial and temporal distribution
ISSN号0147-6513
英文摘要Atmospheric fine particle (PM2.5) samples were collected over a whole year (April 2016 - March 2017) across five sampling locations in the Beijing-Tianjin-Hebei (BTH) region, to investigate the occurrence of novel brominated flame retardants (NBFRs) and polybrominated diphenyl ethers (PBDEs). The concentrations of Sigma(9)NBFRs were in the range of 0.63-104 pg/m(3) (15.6 +/- 16.8 pg/m(3)) in atmospheric PM2.5, while the levels of Sigma 9PBDEs (excluding BDE-209) ranged from 0.05 to 19.1 pg/m(3) (2.9 +/- 3.8 pg/m(3)) and BDE-209 concentrations ranged from 0.88 to 138 pg/m(3) (22 +/- 28 pg/m(3)). Relatively higher levels of NBFRs and PBDEs were found at urban sampling sites in Beijing City and Shijiazhuang City. Decabromodiphenylethane (DBDPE) and BDE-209 were the dominant compounds with the relative abundances of 72% in Sigma(9)NBFRs and 90% in Sigma 10PBDEs, respectively. Generally, the levels of most target BFRs in summer were lower than those in other seasons. However, there were no notable seasonal differences in levels of DBDPE and BDE-209 in atmospheric PM2.5 samples across the BTH region. Significant and positive correlations were found between the concentrations of BFRs and PM2.5. Daily human exposure via inhalation revealed that children have a higher probability of suffering from the adverse effects of BFRs than that of adults. In addition, residents living near sampling locations across the BTH region may suffer high exposure risks to BDE-209 and NBFRs.
内容类型期刊论文
源URL[http://ir.rcees.ac.cn/handle/311016/42910]  
专题生态环境研究中心_环境化学与生态毒理学国家重点实验室
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
2.Shenzhen Ctr Dis Control & Prevent, Shenzhen 518055, Peoples R China
3.Jianghan Univ, Inst Environm & Hlth, Wuhan 430056, Peoples R China
4.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Chem & Ecotoxicol, Beijing 100085, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Weiwei,Wang, Pu,Zhu, Ying,et al. Brominated flame retardants in atmospheric fine particles in the Beijing-Tianjin-Hebei region, China: Spatial and temporal distribution and human exposure assessment[J]. ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY,2019,171:181-189.
APA Zhang, Weiwei.,Wang, Pu.,Zhu, Ying.,Yang, Ruiqiang.,Li, Yingming.,...&Jiang, Guibin.(2019).Brominated flame retardants in atmospheric fine particles in the Beijing-Tianjin-Hebei region, China: Spatial and temporal distribution and human exposure assessment.ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY,171,181-189.
MLA Zhang, Weiwei,et al."Brominated flame retardants in atmospheric fine particles in the Beijing-Tianjin-Hebei region, China: Spatial and temporal distribution and human exposure assessment".ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY 171(2019):181-189.
个性服务
查看访问统计
相关权益政策
暂无数据
收藏/分享
所有评论 (0)
暂无评论
 

除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。


©版权所有 ©2017 CSpace - Powered by CSpace