Realizing High-Ranged Out-of-Plane ZTs in N-Type SnSe Crystals through Promoting Continuous Phase Transition
Chang, C; Wang, DY; He, DS; He, WK; Zhu, FY; Wang, GT; He, JQ; Zhao, LD
刊名ADVANCED ENERGY MATERIALS
2019
卷号9期号:28页码:-
关键词THERMOELECTRIC PERFORMANCE ENHANCEMENT EFFICIENCY FIGURE
ISSN号1614-6832
DOI10.1002/aenm.201901334
文献子类期刊论文
英文摘要Thermoelectric technology enables direct conversion between heat and electricity. The conversion efficiency of a thermoelectric device is determined by the average dimensionless figure of merit ZT(ave). Here, a record high ZT(ave) of approximate to 1.34 in the range of 300-723 K in n-type SnSe based crystals is reported. The remarkable thermoelectric performance derives from the high power factor and the reduced thermal conductivity in the whole temperature range. The high power factor is realized by promoting the continuous phase transition in SnSe crystals through alloying PbSe, which results in a higher symmetry of the crystal structure and the correspondingly modified electronic band structure. Moreover, PbSe alloying induces mass and strain fluctuations, which enables the suppression of thermal transport. These findings provide a new strategy to enhance the thermoelectric performance for the continuous phase transition materials.
语种英语
内容类型期刊论文
源URL[http://ir.sinap.ac.cn/handle/331007/32179]  
专题上海应用物理研究所_中科院上海应用物理研究所2011-2017年
作者单位1.Southern Univ Sci & Technol, Shenzhen Key Lab Thermoelect Mat, Shenzhen 518055, Peoples R China;
2.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201204, Peoples R China;
3.Henan Normal Univ, Coll Phys & Mat Sci, Xinxiang 453007, Henan, Peoples R China
4.Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China;
5.Southern Univ Sci & Technol, Dept Phys, Shenzhen 518055, Peoples R China;
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Chang, C,Wang, DY,He, DS,et al. Realizing High-Ranged Out-of-Plane ZTs in N-Type SnSe Crystals through Promoting Continuous Phase Transition[J]. ADVANCED ENERGY MATERIALS,2019,9(28):-.
APA Chang, C.,Wang, DY.,He, DS.,He, WK.,Zhu, FY.,...&Zhao, LD.(2019).Realizing High-Ranged Out-of-Plane ZTs in N-Type SnSe Crystals through Promoting Continuous Phase Transition.ADVANCED ENERGY MATERIALS,9(28),-.
MLA Chang, C,et al."Realizing High-Ranged Out-of-Plane ZTs in N-Type SnSe Crystals through Promoting Continuous Phase Transition".ADVANCED ENERGY MATERIALS 9.28(2019):-.
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