Loading of Zn/ZnO particles in the precursor feedstock affects the characteristics of liquid plasma sprayed nano-ZnO coatings for photocatalytic applications
Chen, Kuan; Liu, Yi; Fu, Yaoyao; Huang, Jing; Feng, Xiaohua; Wang, Jiang; Zhai, Mengjiao; Lupoi, Rocco; Yin, Shuo; Li, Hua
刊名NANOTECHNOLOGY
2020
卷号31期号:18
关键词ZINC-OXIDE FILMS GAS-SENSING PROPERTIES THIN-FILMS GREEN PHOTOLUMINESCENCE DIFFERENT MORPHOLOGIES NANOSTRUCTURES DEGRADATION MICROSTRUCTURE LUMINESCENCE OXYGEN
DOI10.1088/1361-6528/ab6cda
英文摘要It is known that ZnO is an n-type semiconductor with photocatalytic performances under ultraviolet light irradiation. Constructing a superior structure for a modified electron band has been one of the major research goals for photocatalytic ZnO. Here we report a new technical route for making nano-ZnO coatings with a porous topographic morphology. The coatings were fabricated by plasma spraying the mixture of suspension and solution liquid precursors. Pre-loading of ZnO and Zn powders in the precursor was carried out for the purpose of tailoring the structure of the coatings. The coatings in micron thicknesses showed a porous skeleton and a fluffy top layer consisting of ultrafine ZnO grains. Photocatalytic testing by measuring the degradation of methylene blue revealed significantly enhanced activities of the coatings deposited using the ZnO/Zn loaded precursor. The hybrid-structured ZnO coatings exhibited a narrowed band gap and modified oxygen defects as compared to those deposited from the single liquid feedstock. The results shed light on a one-step easy thermal spray fabrication of polytropic nanostructured functional coatings by employing solid powder-loaded liquid as the starting feedstock.
学科主题Science & Technology - Other Topics ; Materials Science ; Physics
内容类型期刊论文
源URL[http://ir.nimte.ac.cn/handle/174433/19706]  
专题2020专题
作者单位1.Li, H (corresponding author), Chinese Acad Sci, Zhejiang Key Lab Marine Mat & Protect Technol, Ningbo Inst Mat Technol & Engn, Key Lab Marine Mat & Related Technol, Ningbo 315201, Peoples R China.
2.Liu, Y
3.Li, H (corresponding author), Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Cixi Inst Biomed Engn, Ningbo 315201, Peoples R China.
推荐引用方式
GB/T 7714
Chen, Kuan,Liu, Yi,Fu, Yaoyao,et al. Loading of Zn/ZnO particles in the precursor feedstock affects the characteristics of liquid plasma sprayed nano-ZnO coatings for photocatalytic applications[J]. NANOTECHNOLOGY,2020,31(18).
APA Chen, Kuan.,Liu, Yi.,Fu, Yaoyao.,Huang, Jing.,Feng, Xiaohua.,...&Li, Hua.(2020).Loading of Zn/ZnO particles in the precursor feedstock affects the characteristics of liquid plasma sprayed nano-ZnO coatings for photocatalytic applications.NANOTECHNOLOGY,31(18).
MLA Chen, Kuan,et al."Loading of Zn/ZnO particles in the precursor feedstock affects the characteristics of liquid plasma sprayed nano-ZnO coatings for photocatalytic applications".NANOTECHNOLOGY 31.18(2020).
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