Light absorption and emissions inventory of humic-like substances from simulated rainforest biomass burning in Southeast Asia

doi:10.1016/j.envpol.2020.114266

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 中科院海岸带环境过程与生态修复重点实验室 > 近岸生态与环境实验室

	Light absorption and emissions inventory of humic-like substances from simulated rainforest biomass burning in Southeast Asia
	Tang, Jiao 1,2,6; Li, Jun 1,2; Mo, Yangzhi 1,2; Khorram, Mahdi Safaei 1,2; Chen, Yingjun 3; Tang, Jianhui 4; Zhang, Yanlin 5; Song, Jianzhong 1,2; Zhang, Gan 1,2
刊名	ENVIRONMENTAL POLLUTION
	2020-07-01
卷号	262 页码:10
关键词	Brown carbon Mass absorption efficiency Emission factors Regional emissions
ISSN号	0269-7491
DOI	10.1016/j.envpol.2020.114266
通讯作者	Zhang, Gan(zhanggan@gig.ac.cn)
英文摘要	Humic-like substances (HULIS) are complex mixtures that are highly associated with brown carbon (BrC) and are important components of biomass burning (BB) emissions. In this study, we investigated the light absorption, emission factors (EFs), and amounts of HULIS emitted from the simulated burning of 27 types of regionally important rainforest biomass in Southeast Asia. We observed that HULIS had a high mass absorption efficiency at 365 nm (MAE(365)), with an average value of 2.6 +/- 0.83 m(2) g(-1) C. HULIS emitted from BB accounted for 65% +/- 13% of the amount of water-soluble organic carbon (WSOC) and 85% +/- 10% of the light absorption of WSOC at 365 nm. The EFs of HULIS from BB averaged 2.3 +/- 2.1 g kg(-1) fuel, and the burning of the four vegetation subtypes (herbaceous plants, shrubs, evergreen trees, and deciduous trees) exhibited different characteristics. The differences in EFs among the subtypes were likely due to differences in lignin content in the vegetation, the burning conditions, or other factors. The light absorption characteristics of HULIS were strongly associated with the EFs. The annual emissions (minimum-maximum) of HULIS from BB in this region in 2016 were 200-371 Gg. Furthermore, the emissions from January to April accounted for 99% of the total annual emissions of HULIS, which is likely the result of the burning activities during this season. The most significant emission regions were Cambodia, Burma, Thailand, and Laos. This study, which evaluated emissions of HULIS by simulating open BB, contributes to a better understanding of the light-absorbing properties and regional budgets of BrC in this region. (C) 2020 Elsevier Ltd. All rights reserved.
资助项目	Natural Science Foundation of China (NSFC)[41430645] ; Natural Science Foundation of China (NSFC)[41773120] ; National Key R&D Program of China[2017YFC0212000] ; International Partnership Program of Chinese Academy of Sciences[132744KYSB20170002] ; Guangdong Foundation for Program of Science and Technology Research[2017B030314057]
WOS关键词	SOLUBLE ORGANIC-MATTER ; PEARL RIVER DELTA ; OPTICAL-PROPERTIES ; BROWN CARBON ; CHEMICAL-CHARACTERIZATION ; MOLECULAR CHARACTERIZATION ; LIQUID-CHROMATOGRAPHY ; ATMOSPHERIC AEROSOLS ; ANGSTROM EXPONENT ; BLACK CARBON
WOS研究方向	Environmental Sciences & Ecology
语种	英语
WOS记录号	WOS:000533524300095
资助机构	Natural Science Foundation of China (NSFC) ; National Key R&D Program of China ; International Partnership Program of Chinese Academy of Sciences ; Guangdong Foundation for Program of Science and Technology Research
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/29086]
专题	烟台海岸带研究所_近岸生态与环境实验室烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
通讯作者	Zhang, Gan
作者单位	1.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Peoples R China 2.Chinese Acad Sci, Guangdong Key Lab Environm Protect & Resources Ut, Guangzhou Inst Geochem, Guangzhou 510640, Peoples R China 3.Fudan Univ, Dept Environm Sci & Engn, Shanghai 200092, Peoples R China 4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China 5.Nanjing Univ Informat Sci & Technol, Yale NUIST Ctr Atmospher Environm, Nanjing 210044, Peoples R China 6.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Tang, Jiao,Li, Jun,Mo, Yangzhi,et al. Light absorption and emissions inventory of humic-like substances from simulated rainforest biomass burning in Southeast Asia[J]. ENVIRONMENTAL POLLUTION,2020,262:10.
APA	Tang, Jiao.,Li, Jun.,Mo, Yangzhi.,Khorram, Mahdi Safaei.,Chen, Yingjun.,...&Zhang, Gan.(2020).Light absorption and emissions inventory of humic-like substances from simulated rainforest biomass burning in Southeast Asia.ENVIRONMENTAL POLLUTION,262,10.
MLA	Tang, Jiao,et al."Light absorption and emissions inventory of humic-like substances from simulated rainforest biomass burning in Southeast Asia".ENVIRONMENTAL POLLUTION 262(2020):10.