Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China

doi:10.1016/j.envpol.2018.08.011

CORC > 烟台海岸带研究所 > 中国科学院烟台海岸带研究所 > 中科院海岸带环境过程与生态修复重点实验室 > 近岸生态与环境实验室

	Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China
	Liang, Xiaoxue ; Tian, Chongguo ; Zong, Zheng ; Wang, Xiaoping ; Jiang, Wanyanhan ; Chen, Yingjun ; Ma, Jianmin ; Luo, Yongming ; Li, Jun ; Zhang, Gan
刊名	ENVIRONMENTAL POLLUTION
	2018-11
卷号	242 期号:B 页码:1353-1361
关键词	Source-sink relationship Heavy metals Arsenic Water exchange Bohai sea North Yellow sea
ISSN号	0269-7491
DOI	10.1016/j.envpol.2018.08.011
产权排序	[Liang, Xiaoxue ; Jiang, Wanyanhan ; Ma, Jianmin] Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China ; [Tian, Chongguo ; Zong, Zheng ; Luo, Yongming] Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China ; [Zong, Zheng ; Li, Jun ; Zhang, Gan] Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China ; [Wang, Xiaoping] Ludong Univ, Yantai 264025, Peoples R China ; [Chen, Yingjun] Tongji Univ, Coll Environm Sci & Engn, Key Lab Cities Mitigat & Adaptat Climate Change S, Shanghai 200092, Peoples R China ; [Ma, Jianmin] Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
文献子类	Article
英文摘要	This study conducted a field campaign to collect atmospheric deposition samples of heavy metals and arsenic, a metalloid element with typical chemical-physical characteristics (HMA), from 12 sampling sites and water samples from 37 rivers across the Bohai Sea (BS) and North Yellow Sea (NYS) in China. The HMA budgets in the BS and NYS were quantified by a budget model, which was developed based on the HMA inputs from atmospheric deposition and riverine discharge, sequestration to sediment, and interexchange among the BS's four subareas and the NYS. Statistical analyses of 76 deposition samples and 109 water concentration samples showed that atmospheric deposition was a main pathway of Pb entering the BS and NYS, whereas riverine discharge dominated the input of Cr, Cu, Zn, Cd, and As into the marine environment. Modeled results showed that the fractions of HMA in the water bodies compared with their total burdens were 86.6 +/- 4.55% in the Liaodong Bay, 60.5 +/- 10.5% in the Bohai Bay, 20.9 +/- 9.05% in the Laizhou Bay, 95.1 +/- 2.06% in the Central BS, and 94.3 +/- 1.93% in the NYS. The lowest fraction of HMA in the Laizhou Bay was attributed to high sedimentation rates and higher suspended particulate matter concentrations due to inputs from the Yellow River. The modeled 1-, 10- and 100- year mass budgets indicated that the Liaodong Bay in the north of the BS was a sink of HMA, the Bohai Bay and Laizhou Bay in the west and south of the BS acted as sources, and the Central BS and NYS were a transition area for most HMA. (C) 2018 Elsevier Ltd. All rights reserved.
WOS关键词	REGIONAL BACKGROUND SITE ; PEARL RIVER DELTA ; NORTH CHINA ; ATMOSPHERIC DEPOSITION ; SPATIAL-DISTRIBUTION ; LAIZHOU BAY ; CONTAMINATION ASSESSMENT ; PETROLEUM HYDROCARBON ; SURFACE SEDIMENTS ; RISK-ASSESSMENT
WOS研究方向	Environmental Sciences
语种	英语
WOS记录号	WOS:000446282600035
资助机构	Strategic Priority Research Program of the CAS [XDA11020402] ; Natural Scientific Foundation of China [41471413]
内容类型	期刊论文
源URL	[http://ir.yic.ac.cn/handle/133337/24560]
专题	烟台海岸带研究所_近岸生态与环境实验室烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
作者单位	1.Tongji Univ, Coll Environm Sci & Engn, Key Lab Cities Mitigat & Adaptat Climate Change S, Shanghai 200092, Peoples R China; 2.Ludong Univ, Yantai 264025, Peoples R China; 3.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Organ Geochem, Guangzhou 510640, Guangdong, Peoples R China; 4.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China; 5.Lanzhou Univ, Coll Earth & Environm Sci, Key Lab Environm Pollut Predict & Control, Lanzhou 730000, Gansu, Peoples R China; 6.Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
推荐引用方式 GB/T 7714	Liang, Xiaoxue,Tian, Chongguo,Zong, Zheng,et al. Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China[J]. ENVIRONMENTAL POLLUTION,2018,242(B):1353-1361.
APA	Liang, Xiaoxue.,Tian, Chongguo.,Zong, Zheng.,Wang, Xiaoping.,Jiang, Wanyanhan.,...&Zhang, Gan.(2018).Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China.ENVIRONMENTAL POLLUTION,242(B),1353-1361.
MLA	Liang, Xiaoxue,et al."Flux and source-sink relationship of heavy metals and arsenic in the Bohai Sea, China".ENVIRONMENTAL POLLUTION 242.B(2018):1353-1361.