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	Degradation and mineralization of ciprofloxacin by gas-liquid discharge non-thermal plasma
	Hu, Shuheng1,4; Liu, Xinghao1,3,4; Xu, Zimu1,2,4,5; Wang, Jiaquan1; Li, Yunxia1; Shen, Jie2,3,5; Lan, Yan2,3,5; Cheng, Cheng2,3,5
刊名	PLASMA SCIENCE & TECHNOLOGY
	2019
卷号	21期号:1页码:11
关键词	gas-liquid plasma ciprofloxacin mineralization degradation mechanism
ISSN号	1009-0630
DOI	10.1088/2058-6272/aade82
通讯作者	Xu, Zimu(xzm666@hfut.edu.cn) ; Cheng, Cheng(chengcheng@ipp.ac.cn)
英文摘要	A typical quinolones antibiotic ciprofloxacin (CIP) in aqueous solution was degraded by a gas-liquid discharge non-thermal plasma system. The discharge plasma power and the emission intensity of the excited reactive species (RS) generated in the gas phase were detected by the oscilloscope and the optical emission spectroscopy. The effects of various parameters on CIP degradation, i.e. input powers, initial concentrations addition of radical scavengers and pH values were investigated. With the increase of discharge power, the degradation efficiency increased but the energy efficiency significantly reduced. The degradation efficiency also reduced under high concentration of initial CIP conditions due to the competitive reactions between the plasma-induced RS with the degradation intermediates of CIP. Different radical scavengers (isopropanol and CCl4) on center dot OH and H center dot were added into the reaction system and the oxidation effects of center dot OH radicals have been proved with high degradation capacity on CIP. Moreover, the long-term degradation effect on CIP in the plasma-treated aqueous solution proved that the long-lived RS (H2O2 and O-3, etc) might play key roles on the stay effect through multiple aqueous reactions leading to production of center dot OH. The degradation intermediates were determined by the method of electrospray ionization (+)-mass spectroscopy, and the possible degradation mechanism were presented.
资助项目	National Natural Science Foundation of China[51777206] ; National Natural Science Foundation of China[51541807] ; Natural Science Foundation of Anhui Province[1708085MB47] ; Natural Science Foundation of Anhui Province[1708085MA13] ; Foundation of Anhui Province Key Laboratory of Medical Physics and Technology[LMPT2017Y7BP0U1581] ; Doctoral Fund of Ministry of Education of China[2017M612058] ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology[JZ2016HGBZ0768] ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology[JZ2016HGBZ0769] ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology[JZ2017HGBZ0944]
WOS关键词	DIELECTRIC BARRIER DISCHARGE ; PERSONAL CARE PRODUCTS ; PHOTO-FENTON PROCESS ; AQUEOUS-SOLUTION ; WASTE-WATER ; HYDROXYL RADICALS ; OXIDATION-PRODUCTS ; REACTION-KINETICS ; DRINKING-WATER ; RATE CONSTANTS
WOS研究方向	Physics
语种	英语
出版者	IOP PUBLISHING LTD
WOS记录号	WOS:000450187600001
资助机构	National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; 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Specialized Research Fund for the Doctoral Program of Hefei University of Technology ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology ; Specialized Research Fund for the Doctoral Program of Hefei University of Technology
内容类型	期刊论文
源URL	[http://ir.hfcas.ac.cn:8080/handle/334002/34139]
专题	合肥物质科学研究院_中科院等离子体物理研究所
通讯作者	Xu, Zimu; Cheng, Cheng
作者单位	1.Hefei Univ Technol, Sch Resources & Environm Engn, Hefei 230009, Anhui, Peoples R China 2.Chinese Acad Sci, Ctr Med Phys & Technol, Hefei Inst Phys Sci, Hefei 230031, Anhui, Peoples R China 3.Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China 4.Hefei Univ Technol, Intelligent Mfg Technol Res Inst, Hefei 230088, Anhui, Peoples R China 5.Chinese Acad Sci, Hefei Inst Phys Sci, Anhui Prov Key Lab Med Phys & Technol, Hefei 230031, Anhui, Peoples R China
推荐引用方式 GB/T 7714	Hu, Shuheng,Liu, Xinghao,Xu, Zimu,et al. Degradation and mineralization of ciprofloxacin by gas-liquid discharge non-thermal plasma[J]. PLASMA SCIENCE & TECHNOLOGY,2019,21(1):11.
APA	Hu, Shuheng.,Liu, Xinghao.,Xu, Zimu.,Wang, Jiaquan.,Li, Yunxia.,...&Cheng, Cheng.(2019).Degradation and mineralization of ciprofloxacin by gas-liquid discharge non-thermal plasma.PLASMA SCIENCE & TECHNOLOGY,21(1),11.
MLA	Hu, Shuheng,et al."Degradation and mineralization of ciprofloxacin by gas-liquid discharge non-thermal plasma".PLASMA SCIENCE & TECHNOLOGY 21.1(2019):11.

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