Immobilization of simulated An(4+) in radioactive contaminated clay via microwave sintering
Shu, Xiaoyan1,3,8; Chen, Shunzhang1,2; Huang, Wenxiao4; Li, Bingsheng3,8; Shao, Dadong5; Xie, Yi6,7; Lu, Xirui1,3,8
刊名MATERIALS CHEMISTRY AND PHYSICS
2020-11-01
卷号254
关键词Radioactive contaminated soil Immobilization Glass composite material Microwave sintering Chemical durability
ISSN号0254-0584
DOI10.1016/j.matchemphys.2020.123534
通讯作者Lu, Xirui(luxirui@swust.edu.cn)
英文摘要To rapidly immobilize simulated An(4+) in high-alumina soil by microwave sintering, clay sample doped with 5 wt % of CeO2 was successfully fabricated as silicate glass composite matrix at 1500 degrees C in 30 min Ce4+ was immobilized into glass phase, which was formed through the reaction of feldspar and quartz. The generated crystal phase Al6Si2O13 in sintered glass composite material was due to the formation of [Si2O7](6-) groups, which were separated from the glass network structure. The leaching rate of Ce maintained at a magnitude of 1 x 10(-7) g.m(-2) d(-1) after 42 days for all samples. Moreover, increased sintering temperature is beneficial to enhance the leaching resistance of sintered clay samples.
资助项目National Natural Science Foundation of China[21677118] ; Longshan academic talent research supporting program of SWUST[18LZX312] ; Longshan academic talent research supporting program of SWUST[18LZX520] ; State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology[18fksy0213]
WOS关键词SOIL ; FTIR ; FUKUSHIMA ; RAMAN
WOS研究方向Materials Science
语种英语
出版者ELSEVIER SCIENCE SA
WOS记录号WOS:000570092100004
资助机构National Natural Science Foundation of China ; Longshan academic talent research supporting program of SWUST ; State Key Laboratory of Environment-friendly Energy Materials, Southwest University of Science and Technology
内容类型期刊论文
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/104091]  
专题中国科学院合肥物质科学研究院
通讯作者Lu, Xirui
作者单位1.Southwest Univ Sci & Technol, Fundamental Sci Nucl Wastes & Environm Safety Lab, Mianyang 621010, Sichuan, Peoples R China
2.Sichuan Univ, Key Lab Radiat Phys & Technol, Minist Educ, Inst Nucl Sci & Technol, Chengdu 610064, Peoples R China
3.Southwest Univ Sci & Technol, Natl Coinnovat Ctr Nucl Waste Disposal & Environm, Mianyang 621010, Sichuan, Peoples R China
4.Minist Land & Resources, Key Lab Radioact & Rare Scattered Minerals, Shaoguan 512026, Peoples R China
5.Nanjing Univ Sci & Technol, Nanjing 210094, Jiangsu, Peoples R China
6.Univ Sci & Technol China, Hefei 230026, Peoples R China
7.Chinese Acad Sci, Inst Plasma Phys, CAS Key Lab Photovolta & Energy Conservat Mat, POB 1126, Hefei 230031, Peoples R China
8.Southwest Univ Sci & Technol, State Key Lab Environm Friendly Energy Mat, Mianyang 621010, Sichuan, Peoples R China
推荐引用方式
GB/T 7714
Shu, Xiaoyan,Chen, Shunzhang,Huang, Wenxiao,et al. Immobilization of simulated An(4+) in radioactive contaminated clay via microwave sintering[J]. MATERIALS CHEMISTRY AND PHYSICS,2020,254.
APA Shu, Xiaoyan.,Chen, Shunzhang.,Huang, Wenxiao.,Li, Bingsheng.,Shao, Dadong.,...&Lu, Xirui.(2020).Immobilization of simulated An(4+) in radioactive contaminated clay via microwave sintering.MATERIALS CHEMISTRY AND PHYSICS,254.
MLA Shu, Xiaoyan,et al."Immobilization of simulated An(4+) in radioactive contaminated clay via microwave sintering".MATERIALS CHEMISTRY AND PHYSICS 254(2020).
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