Reduced-Dimensional Perovskite Enabled by Organic Diamine for Efficient Photovoltaics | |
Niu, TT; Ren, H; Wu, B; Xia, YD; Xie, XJ; Yang, YG; Gao, XY; Chen, YH; Huang, W | |
刊名 | JOURNAL OF PHYSICAL CHEMISTRY LETTERS
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2019 | |
卷号 | 10期号:10页码:2349—2356 |
关键词 | POLYMER SOLAR-CELLS ADVANTAGES MIGRATION |
ISSN号 | 1948-7185 |
DOI | 10.1021/acs.jpclett.9b00750 |
文献子类 | 期刊论文 |
英文摘要 | Reduced-dimensional (RD) perovskite solar cells (PSCs) are emerging as highly attractive alternatives to three-dimensional (3D) PSCs due to their dramatically improved environmental stability and photostability. Diamine-based RD perovskites with a single organic amine interlayer possess orderly inorganic sheets and a smaller insulation area, indicating great potential in combining high efficiency and long-term stability. Here, we report an efficient and stable RD PSC based on 1,4-butanediamine (BDA). We found that the BDA-based RD perovskite exhibits improved crystallinity, reduced trap-state densities, and enhanced charge mobility compared to those of butylamine (BA)-based RD (BA-RD) perovskite. A high power conversion efficiency of 17.91% was achieved with negligible hysteresis. Moreover, the device showed improved stability compared to those of BA-RD and 3D films and devices. The findings may inspire new developments in introducing organic diamine for efficient and stable RD PSCs. |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.sinap.ac.cn/handle/331007/31796] ![]() |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
作者单位 | 1.Nanjing Univ Posts & Telecommun, KLOEID, 9 Wenyuan Rd, Nanjing 210023, Jiangsu, Peoples R China; 2.Nanjing Tech Univ NanjingTech, Jiangsu Natl Synergist Innovat Ctr Adv Mat SICAM, Key Lab Flexible Elect KLOFE, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China; 3.Nanjing Tech Univ NanjingTech, Jiangsu Natl Synergist Innovat Ctr Adv Mat SICAM, IAM, 30 South Puzhu Rd, Nanjing 211816, Jiangsu, Peoples R China; 4.Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, 21 Nanyang Link, Singapore 637371, Singapore; 5.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai Synchrotron Radiat Facil, Shanghai 201204, Peoples R China; 6.NPU, SIFE, 127 West Youyi Rd, Xian 710072, Shaanxi, Peoples R China; 7.Nanjing Univ Posts & Telecommun, IAM, 9 Wenyuan Rd, Nanjing 210023, Jiangsu, Peoples R China |
推荐引用方式 GB/T 7714 | Niu, TT,Ren, H,Wu, B,et al. Reduced-Dimensional Perovskite Enabled by Organic Diamine for Efficient Photovoltaics[J]. JOURNAL OF PHYSICAL CHEMISTRY LETTERS,2019,10(10):2349—2356. |
APA | Niu, TT.,Ren, H.,Wu, B.,Xia, YD.,Xie, XJ.,...&Huang, W.(2019).Reduced-Dimensional Perovskite Enabled by Organic Diamine for Efficient Photovoltaics.JOURNAL OF PHYSICAL CHEMISTRY LETTERS,10(10),2349—2356. |
MLA | Niu, TT,et al."Reduced-Dimensional Perovskite Enabled by Organic Diamine for Efficient Photovoltaics".JOURNAL OF PHYSICAL CHEMISTRY LETTERS 10.10(2019):2349—2356. |
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