Sustainable Synthesis of Pure Silica Zeolites from a Combined Strategy of Zeolite Seeding and Alcohol Filling
Wu, Qinming3; Zhu, Longfeng3,4; Chu, Yueying2; Liu, Xiaolong2; Zhang, Changsheng3; Zhang, Juan3; Xu, Hao3; Xu, Jun2; Deng, Feng2; Feng, Zhaochi1
刊名ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
2019-07-30
页码6
关键词seeding silica sustainable synthesis zeolites
ISSN号1433-7851
DOI10.1002/anie.201906559
英文摘要Currently, the synthesis of pure silica zeolites always requires the presence of organic structure-directing agents (OSDAs), which direct the assembly pathway and ultimately fill the pore space. A sustainable route is now reported for synthesizing pure silica zeolites in the absence of OSDAs from a combined strategy of zeolite seeding and alcohol filling, where the zeolite seeds direct crystallization of zeolite crystals from amorphous silica, while the alcohol is served as pore filling in the zeolites. Very importantly, the alcohol could be fully washed out from zeolite pores by water at room temperature, which completely avoids calcination at high temperature for removal of OSDAs in the synthesis of pure silica zeolites.
资助项目National Key Research and Development Program of China[2017YFB0702803] ; National Natural Science Foundation of China[21703203] ; National Natural Science Foundation of China[21802053] ; National Natural Science Foundation of China[21673282] ; National Natural Science Foundation of China[21673205]
WOS关键词ORGANOTEMPLATE-FREE ; DIRECTING AGENT ; CRYSTALLIZATION ; GROWTH ; ZSM-5
WOS研究方向Chemistry
语种英语
出版者WILEY-V C H VERLAG GMBH
WOS记录号WOS:000479615700001
资助机构National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China
内容类型期刊论文
源URL[http://ir.wipm.ac.cn/handle/112942/14847]  
专题中国科学院武汉物理与数学研究所
通讯作者Wu, Qinming; Deng, Feng; Xiao, Feng-Shou
作者单位1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China
2.Chinese Acad Sci, State Key Lab Magnet Resonance & Atom & Mol Phys, Wuhan Ctr Magnet Resonance, Wuhan Inst Phys & Math, Wuhan 430071, Hubei, Peoples R China
3.Zhejiang Univ, Dept Chem, Hangzhou 310007, Zhejiang, Peoples R China
4.Jiaxing Univ, Coll Biol Chem Sci & Engn, Jiaxing 314001, Peoples R China
推荐引用方式
GB/T 7714
Wu, Qinming,Zhu, Longfeng,Chu, Yueying,et al. Sustainable Synthesis of Pure Silica Zeolites from a Combined Strategy of Zeolite Seeding and Alcohol Filling[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2019:6.
APA Wu, Qinming.,Zhu, Longfeng.,Chu, Yueying.,Liu, Xiaolong.,Zhang, Changsheng.,...&Xiao, Feng-Shou.(2019).Sustainable Synthesis of Pure Silica Zeolites from a Combined Strategy of Zeolite Seeding and Alcohol Filling.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,6.
MLA Wu, Qinming,et al."Sustainable Synthesis of Pure Silica Zeolites from a Combined Strategy of Zeolite Seeding and Alcohol Filling".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019):6.
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