Confinement Catalysis with 2D Materials for Energy Conversion

doi:10.1002/adma.201901996

	Confinement Catalysis with 2D Materials for Energy Conversion
	Tang, Lei 1,2; Meng, Xianguang 1; Deng, Dehui 1,2; Bao, Xinhe 1,2
刊名	ADVANCED MATERIALS
	2019-08-07
页码	16
关键词	2D materials confinement catalysis energy conversion single atoms
ISSN号	0935-9648
DOI	10.1002/adma.201901996
通讯作者	Deng, Dehui(dhdeng@dicp.ac.cn)
英文摘要	The unique electronic and structural properties of 2D materials have triggered wide research interest in catalysis. The lattice of 2D materials and the interface between 2D covers and other substrates provide intriguing confinement environments for active sites, which has stimulated a rising area of "confinement catalysis with 2D materials." Fundamental understanding of confinement catalysis with 2D materials will favor the rational design of high-performance 2D nanocatalysts. Confinement catalysis with 2D materials has found extensive applications in energy-related reaction processes, especially in the conversion of small energy-related molecules such as O-2, CH4, CO, CO2, H2O, and CH3OH. Two representative strategies, i.e., 2D lattice-confined single atoms and 2D cover-confined metals, have been applied to construct 2D confinement catalytic systems with superior catalytic activity and stability. Herein, the recent advances in the design, applications, and structure-performance analysis of two 2D confinement catalytic systems are summarized. The different routes for tuning the electronic states of 2D confinement catalysts are highlighted and perspectives on confinement catalysis with 2D materials toward energy conversion and utilization in the future are provided.
资助项目	Ministry of Science and Technology of China[2016YFA0204100] ; Ministry of Science and Technology of China[2016YFA0200200] ; National Natural Science Foundation of China[21890753] ; National Natural Science Foundation of China[21573220] ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences[QYZDB-SSW-JSC020] ; DNL Cooperation Fund, CAS[DNL180201]
WOS关键词	OXYGEN REDUCTION REACTION ; NITROGEN-DOPED GRAPHENE ; ELECTROCATALYTIC HYDROGEN EVOLUTION ; SINGLE-ATOM CATALYSTS ; ACTIVE-SITES ; CARBON NANOTUBES ; 2-DIMENSIONAL MATERIALS ; MOLYBDENUM-DISULFIDE ; EFFICIENT CATALYSTS ; MOS2 NANOSHEETS
WOS研究方向	Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种	英语
出版者	WILEY-V C H VERLAG GMBH
WOS记录号	WOS:000480175300001
资助机构	Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS ; Ministry of Science and Technology of China ; Ministry of Science and Technology of China ; National Natural Science Foundation of China ; National Natural Science Foundation of China ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; Key Research Program of Frontier Sciences of the Chinese Academy of Sciences ; DNL Cooperation Fund, CAS ; DNL Cooperation Fund, CAS
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/173483]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Deng, Dehui
作者单位	1.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Zhongshan Rd 457, Dalian 116023, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
推荐引用方式 GB/T 7714	Tang, Lei,Meng, Xianguang,Deng, Dehui,et al. Confinement Catalysis with 2D Materials for Energy Conversion[J]. ADVANCED MATERIALS,2019:16.
APA	Tang, Lei,Meng, Xianguang,Deng, Dehui,&Bao, Xinhe.(2019).Confinement Catalysis with 2D Materials for Energy Conversion.ADVANCED MATERIALS,16.
MLA	Tang, Lei,et al."Confinement Catalysis with 2D Materials for Energy Conversion".ADVANCED MATERIALS (2019):16.