Microstructural evolution of epitaxial Ti3AlC2 film on sapphire under ion irradiation and nanoindentation-induced deformation
Huang, Qing1; Wang, Ji1; Shao, Tao1; Ren, Donglou1; Liu, Shaoshuai5; Eklund, Per4; Huang, Rong3; Zhu, Yabin2; Huang, Feng1; Du, Shiyu1
刊名JOURNAL OF NUCLEAR MATERIALS
2018-10-01
卷号509页码:181-187
关键词Ion irradiation Accident tolerant fuels Fuel cladding coating Ti3AlC2 MAX phase film
ISSN号0022-3115
DOI10.1016/j.jnucmat.2018.06.045
英文摘要Feasibility of Ti3AlC2 phase as the protective coatings of accident tolerant fuels (ATFs) was investigated by means of ions irradiation, nanoindentation and transmission electron microscopy. Au ions irradiation was carried out on thin Ti3AlC2 film to simulate the high displacement damage induced by the energetic particles in the nuclear reactors. Nanoindentation on the Ti3AlC2 film was followed subsequently as a source of external stress to simulate the high pressure applied on the cladding in nuclear reactor cores of pressurized water reactors (PWRs). TEM was used to characterize the microstructural evolution of Ti3AlC2 film after irradiation and nanoindentation. TEM analysis shows that Ti3AlC2 film remains pristine layered structure and no amorphization was detected after irradiation to similar to 14 dpa. The combined nanoindentation and TEM show that no rupture and exfoliation of the Au-irradiated Ti3AlC2 film occur even the extern stress and total elongation induced by nanoindentation reach to 16.6 GPa and similar to 5%, respectively. The above results show good irradiation resistance and good ductility as well as excellent adhesion of the Ti3AlC2 coating on the substrate after high dose irradiation and under high external stress. This indicates the good feasibility of Ti3AlC2 thin films as the coatings of ATF claddings. (C) 2018 Elsevier B.V. All rights reserved.
资助项目National Natural Science Foundation of China[91226202] ; National Natural Science Foundation of China[91426304] ; National Natural Science Foundation of China[11505247] ; CAS Interdisciplinary Innovation Team
WOS关键词ACCIDENT TOLERANT FUELS ; MAX PHASES ; RADIATION TOLERANCE ; NEUTRON-IRRADIATION ; M(N+1)AX(N) PHASES ; THIN-FILMS ; DEPOSITION ; TI3SIC2 ; TI2ALC ; CERAMICS
WOS研究方向Materials Science ; Nuclear Science & Technology
语种英语
出版者ELSEVIER SCIENCE BV
WOS记录号WOS:000442483300020
资助机构National Natural Science Foundation of China ; CAS Interdisciplinary Innovation Team
内容类型期刊论文
源URL[http://119.78.100.186/handle/113462/59341]  
专题近代物理研究所_先进核能材料研究室(ADS)
通讯作者Huang, Qing
作者单位1.Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Engn Lab Nucl Energy Mat, Ningbo 315201, Zhejiang, Peoples R China
2.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Gansu, Peoples R China
3.East China Normal Univ, Key Lab Polar Mat & Devices, Minist Educ, Shanghai, Peoples R China
4.Linkoping Univ, IFM, Thin Film Phys Div, SE-58183 Linkoping, Sweden
5.Peking Univ, Ctr Appl Phys & Technol, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China
推荐引用方式
GB/T 7714
Huang, Qing,Wang, Ji,Shao, Tao,et al. Microstructural evolution of epitaxial Ti3AlC2 film on sapphire under ion irradiation and nanoindentation-induced deformation[J]. JOURNAL OF NUCLEAR MATERIALS,2018,509:181-187.
APA Huang, Qing.,Wang, Ji.,Shao, Tao.,Ren, Donglou.,Liu, Shaoshuai.,...&Wang, Yugang.(2018).Microstructural evolution of epitaxial Ti3AlC2 film on sapphire under ion irradiation and nanoindentation-induced deformation.JOURNAL OF NUCLEAR MATERIALS,509,181-187.
MLA Huang, Qing,et al."Microstructural evolution of epitaxial Ti3AlC2 film on sapphire under ion irradiation and nanoindentation-induced deformation".JOURNAL OF NUCLEAR MATERIALS 509(2018):181-187.
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