DISSOCIATIVE RECOMBINATION MEASUREMENTS OF HCl+ USING AN ION STORAGE RING | |
Novotny, O.1; Becker, A.2; Buhr, H.2; Domesle, C.2; Geppert, W.3; Grieser, M.2; Krantz, C.2; Kreckel, H.2; Repnow, R.2; Schwalm, D.2,4 | |
刊名 | ASTROPHYSICAL JOURNAL
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2013-11-01 | |
卷号 | 777 |
关键词 | Astrochemistry Ism: Clouds Ism: Molecules Methods: Laboratory: Molecular Molecular Data Molecular Processes |
ISSN号 | 0004-637X |
DOI | 10.1088/0004-637X/777/1/54 |
文献子类 | Article |
英文摘要 | We have measured dissociative recombination (DR) of HCl+ with electrons using a merged beams configuration at the TSR heavy-ion storage ring located at the Max Planck Institute for Nuclear Physics in Heidelberg, Germany. We present the measured absolute merged beams recombination rate coefficient for collision energies from 0 to 4.5 eV. We have also developed a new method for deriving the cross section from the measurements. Our approach does not suffer from approximations made by previously used methods. The cross section was transformed to a plasma rate coefficient for the electron temperature range from T = 10 to 5000 K. We show that the previously used HCl+ DR data underestimate the plasma rate coefficient by a factor of 1.5 at T = 10 K and overestimate it by a factor of three at T = 300 K. We also find that the new data may partly explain existing discrepancies between observed abundances of chlorine-bearing molecules and their astrochemical models. |
资助项目 | COST Action[CM0805] |
WOS关键词 | HIGH-RESOLUTION MEASUREMENT ; CHLORINE-BEARING MOLECULES ; DENSE INTERSTELLAR CLOUDS ; DIELECTRONIC-RECOMBINATION ; HYDROGEN-CHLORIDE ; HERSCHEL/HIFI DISCOVERY ; BEAM ; TSR ; PHOTODISSOCIATION ; PREDISSOCIATION |
WOS研究方向 | Astronomy & Astrophysics |
语种 | 英语 |
出版者 | IOP PUBLISHING LTD |
WOS记录号 | WOS:000326147300054 |
内容类型 | 期刊论文 |
源URL | [http://119.78.100.186/handle/113462/48493] ![]() |
专题 | 中国科学院近代物理研究所 |
通讯作者 | Novotny, O. |
作者单位 | 1.Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA 2.Max Planck Inst Nucl Phys, D-69117 Heidelberg, Germany 3.Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden 4.Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel 5.Univ Giessen, Inst Atom & Mol Phys, D-35392 Giessen, Germany 6.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China |
推荐引用方式 GB/T 7714 | Novotny, O.,Becker, A.,Buhr, H.,et al. DISSOCIATIVE RECOMBINATION MEASUREMENTS OF HCl+ USING AN ION STORAGE RING[J]. ASTROPHYSICAL JOURNAL,2013,777. |
APA | Novotny, O..,Becker, A..,Buhr, H..,Domesle, C..,Geppert, W..,...&Savin, D. W..(2013).DISSOCIATIVE RECOMBINATION MEASUREMENTS OF HCl+ USING AN ION STORAGE RING.ASTROPHYSICAL JOURNAL,777. |
MLA | Novotny, O.,et al."DISSOCIATIVE RECOMBINATION MEASUREMENTS OF HCl+ USING AN ION STORAGE RING".ASTROPHYSICAL JOURNAL 777(2013). |
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