Sedimentary records of polychlorinated biphenyls in the East China Marginal Seas and Great Lakes: Significance of recent rise of emissions in China and environmental implications | |
Wu, Zilan1; Lin, Tian2,3; Li, An3; Zhou, Shanshan4; He, Huan3,5; Guo, Jiehong3; Hu, Limin6; Li, Yuanyuan1; Guo, Zhigang1 | |
刊名 | ENVIRONMENTAL POLLUTION |
2019-11 | |
卷号 | 254 |
关键词 | PCBs Sedimentary records ECMSs Great lakes |
ISSN号 | 0269-7491 |
DOI | 10.1016/j.envpol.2019.112972 |
英文摘要 | Polychlorinated biphenyls (PCBs) in dated sediment cores from the East China Marginal Seas (Sigma CMSs) and the chronology of the net fluxes to sediments were analyzed. The accumulation of 27 PCBs (Sigma PCBs) in the ECMS sediments is about 5-26 ng cm(-2), with the net depositional fluxes of Sigma PCBs 10 times lower than those observed in the Great Lakes during the 1960s-1970s. Exponential increases in PCB deposition to the ECMS sediments since the 1990s were observed, which closely follows the fast growth of PCB emissions from industrial thermal processes and e-waste related sources in China. Recent PCB fluxes to the study sites in the ECMSs and the Great Lakes are comparable; the former surged forward with a rising tendency, while the latter showed continued decline after the late 1970s. Due to the different PCB application histories and sources between the two regions, the ECMS sediments may remain as a net sink for land-derived PCBs, while sediments in the Great Lake may have been acting as a secondary source releasing PCBs to water. A higher proportion of trichlorobiphenyls in the ECMS sediments than the Great Lakes was indicated, which may imply the net transport of atmospheric PCBs from China. (C) 2019 Elsevier Ltd. All rights reserved. |
电子版国际标准刊号 | 18736424 |
资助项目 | national water pollution control and management in China[2009ZX07528-002] |
WOS研究方向 | Environmental Sciences & Ecology |
语种 | 英语 |
出版者 | ELSEVIER SCI LTD |
WOS记录号 | WOS:000488887500077 |
内容类型 | 期刊论文 |
源URL | [http://ir.fio.com.cn:8080/handle/2SI8HI0U/30253] |
专题 | 业务部门_海洋地质与地球物理研究室 |
通讯作者 | Lin, Tian |
作者单位 | 1.Fudan Univ, Shanghai Key Lab Atmospher Particle Pollut & Prev, Dept Environm Sci & Engn, Shanghai 200433, Peoples R China 2.Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550081, Guizhou, Peoples R China 3.Univ Illinois, Sch Publ Hlth, Chicago, IL 60612 USA 4.Zhejiang Univ Technol, Coll Environm, Hangzhou 310032, Zhejiang, Peoples R China 5.Nanjing Normal Univ, Sch Environm, Nanjing 210023, Jiangsu, Peoples R China 6.State Ocean Adm, Inst Oceanog 1, Key Lab Marine Sedimentol & Environm Geol, Qingdao 266061, Shandong, Peoples R China |
推荐引用方式 GB/T 7714 | Wu, Zilan,Lin, Tian,Li, An,et al. Sedimentary records of polychlorinated biphenyls in the East China Marginal Seas and Great Lakes: Significance of recent rise of emissions in China and environmental implications[J]. ENVIRONMENTAL POLLUTION,2019,254. |
APA | Wu, Zilan.,Lin, Tian.,Li, An.,Zhou, Shanshan.,He, Huan.,...&Guo, Zhigang.(2019).Sedimentary records of polychlorinated biphenyls in the East China Marginal Seas and Great Lakes: Significance of recent rise of emissions in China and environmental implications.ENVIRONMENTAL POLLUTION,254. |
MLA | Wu, Zilan,et al."Sedimentary records of polychlorinated biphenyls in the East China Marginal Seas and Great Lakes: Significance of recent rise of emissions in China and environmental implications".ENVIRONMENTAL POLLUTION 254(2019). |
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