Mechanochemistry Induced Using Force Exerted by a Functionalized Microscope Tip | |
Zhang, Yajie ; Wang, Yongfeng ; Lu, Jing-Tao ; Brandbyge, Mads ; Berndt, Richard | |
刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
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2017 | |
关键词 | conformation analysis mechanochemistry scanning probe microscopy surface chemistry tin SCANNING TUNNELING MICROSCOPE SINGLE-MOLECULE MANIPULATION STM |
DOI | 10.1002/anie.201704940 |
英文摘要 | Atomic-scale mechanochemistry is realized from force exerted by a C-60-functionalized scanning tunneling microscope tip. Two conformers of tin phthalocyanine can be prepared on coinage-metal surfaces. A transition between these conformers is induced on Cu(111) and Ag(100). Density-functional calculations reveal details of this reaction. Because of the large energy barrier of the reaction and the strong interaction of SnPc with Cu(111), the process cannot be achieved by electrical means.; National Natural Science Foundation of China [21522301, 21373020, 21403008, 61321001, 21433011, 11304107, 61371015]; Ministry of Science and Technology [2014CB239302, 2013CB933404, 2017YFA0205003]; Deutsche Forschungsgemeinschaft [Sonderforschungsbereich 677]; SCI(E); ARTICLE; 39; 11769-11773; 56 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/470828] ![]() |
专题 | 信息科学技术学院 |
推荐引用方式 GB/T 7714 | Zhang, Yajie,Wang, Yongfeng,Lu, Jing-Tao,et al. Mechanochemistry Induced Using Force Exerted by a Functionalized Microscope Tip[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2017. |
APA | Zhang, Yajie,Wang, Yongfeng,Lu, Jing-Tao,Brandbyge, Mads,&Berndt, Richard.(2017).Mechanochemistry Induced Using Force Exerted by a Functionalized Microscope Tip.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION. |
MLA | Zhang, Yajie,et al."Mechanochemistry Induced Using Force Exerted by a Functionalized Microscope Tip".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017). |
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