Dry and wet deposition of inorganic nitrogen compounds to a tropical   pasture site (Rondonia, Brazil)

CORC > 北京大学 > 环境科学与工程学院

	Dry and wet deposition of inorganic nitrogen compounds to a tropical pasture site (Rondonia, Brazil)
	Trebs, I ; Lara, LL ; Zeri, LMM ; Gatti, LV ; Artaxo, P ; Dlugi, R ; Slanina, J ; Andreae, MO ; Meixner, FX
刊名	atmospheric chemistry and physics
	2006
关键词	SURFACE-EXCHANGE FLUXES INTENSIVELY MANAGED GRASSLAND AMMONIA COMPENSATION POINT GAS-PARTICLE INTERACTIONS JET AEROSOL COLLECTOR NITRIC-ACID GRADIENT MEASUREMENTS ATMOSPHERIC NITROGEN AMAZON BASIN PRECIPITATION CHEMISTRY
英文摘要	The input of nitrogen (N) to ecosystems has increased dramatically over the past decades. While total (wet + dry) N deposition has been extensively determined in temperate regions, only very few data sets of N wet deposition exist for tropical ecosystems, and moreover, reliable experimental information about N dry deposition in tropical environments is lacking. In this study we estimate dry and wet deposition of inorganic N for a remote pasture site in the Amazon Basin based on in-situ measurements. The measurements covered the late dry (biomass burning) season, a transition period and the onset of the wet season (clean conditions) (12 September to 14 November 2002) and were a part of the LBA-SMOCC (Large-Scale Biosphere-Atmosphere Experiment in Amazonia-Smoke, Aerosols, Clouds, Rainfall, and Climate) 2002 campaign. Ammonia (NH3), nitric acid (HNO3), nitrous acid (HONO), nitrogen dioxide (NO2), nitric oxide (NO), ozone (O-3), aerosol ammonium (NH4+) and aerosol nitrate (NO3-) were measured in real-time, accompanied by simultaneous meteorological measurements. Dry deposition fluxes of NO2 and HNO3 are inferred using the "big leaf multiple resistance approach" and particle deposition fluxes are derived using an established empirical parameterization. Bi-directional surface-atmosphere exchange fluxes of NH3 and HONO are estimated by applying a "canopy compensation point model". N dry and wet deposition is dominated by NH3 and NH4+, which is largely the consequence of biomass burning during the dry season. The grass surface appeared to have a strong potential for daytime NH3 emission, owing to high canopy compensation points, which are related to high surface temperatures and to direct NH3 emissions from cattle excreta. NO2 also significantly accounted for N dry deposition, whereas HNO3, HONO and N-containing aerosol species were only minor contributors. Ignoring NH3 emission from the vegetation surface, the annual net N deposition rate is estimated to be about -11 kgN ha(-1) yr(-1). If on the other hand, surface-atmosphere exchange of NH3 is considered to be bi-directional, the annual net N budget at the pasture site is estimated to range from -2.15 to -4.25 kgN ha(-1) yr(-1).; Meteorology & Atmospheric Sciences; SCI(E); 0; REVIEW; 447-469; 6
语种	英语
内容类型	期刊论文
源URL	[http://ir.pku.edu.cn/handle/20.500.11897/398769]
专题	环境科学与工程学院
推荐引用方式 GB/T 7714	Trebs, I,Lara, LL,Zeri, LMM,et al. Dry and wet deposition of inorganic nitrogen compounds to a tropical pasture site (Rondonia, Brazil)[J]. atmospheric chemistry and physics,2006.
APA	Trebs, I.,Lara, LL.,Zeri, LMM.,Gatti, LV.,Artaxo, P.,...&Meixner, FX.(2006).Dry and wet deposition of inorganic nitrogen compounds to a tropical pasture site (Rondonia, Brazil).atmospheric chemistry and physics.
MLA	Trebs, I,et al."Dry and wet deposition of inorganic nitrogen compounds to a tropical pasture site (Rondonia, Brazil)".atmospheric chemistry and physics (2006).