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Examining the Impact of Nitrous Acid Chemistry on Ozone and PM over the Pearl River Delta Region
Zhang, Rui ; Sarwar, Golam ; Fung, Jimmy C. H. ; Lau, Alexis K. H. ; Zhang, Yuanhang
刊名advances in meteorology
2012
关键词ATMOSPHERIC BOUNDARY-LAYER AIR-QUALITY WATER-VAPOR NITRIC-ACID HETEROGENEOUS HYDROLYSIS EMISSION INVENTORY HONO FORMATION HUMIC-ACID MODEL NO2
DOI10.1155/2012/140932
英文摘要The impact of nitrous acid (HONO) chemistry on regional ozone and particulate matter in Pearl River Delta region was investigated using the community multiscale air quality (CMAQ) modeling system and the CB05 mechanism. Model simulations were conducted for a ten-day period in October 2004. Compared with available observed data, the model performance for NOx, SO2, PM10, and sulfate is reasonably good; however, predictions of HONO are an order of magnitude lower than observed data. The CB05 mechanism contains several homogenous reactions related to HONO. To improve the model performance for HONO, direct emissions, two heterogeneous reactions, and two surface photolysis reactions were incorporated into the model. The inclusion of the additional formation pathways significantly improved simulated HONO compared with observed data. The addition of HONO sources enhances daily maximum 8-hour ozone by up to 6 ppbV (8%) and daily mean PM2.5 by up to 17 ug/m(3) (12%). They also affected ozone control strategy in Pearl River Delta region.; Meteorology & Atmospheric Sciences; SCI(E); 0; ARTICLE
语种英语
内容类型期刊论文
源URL[http://ir.pku.edu.cn/handle/20.500.11897/393893]  
专题环境科学与工程学院
推荐引用方式
GB/T 7714
Zhang, Rui,Sarwar, Golam,Fung, Jimmy C. H.,et al. Examining the Impact of Nitrous Acid Chemistry on Ozone and PM over the Pearl River Delta Region[J]. advances in meteorology,2012.
APA Zhang, Rui,Sarwar, Golam,Fung, Jimmy C. H.,Lau, Alexis K. H.,&Zhang, Yuanhang.(2012).Examining the Impact of Nitrous Acid Chemistry on Ozone and PM over the Pearl River Delta Region.advances in meteorology.
MLA Zhang, Rui,et al."Examining the Impact of Nitrous Acid Chemistry on Ozone and PM over the Pearl River Delta Region".advances in meteorology (2012).
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