Comparable hydrogen isotopic fractionation of plant leaf wax n-alkanoic   acids in arid and humid subtropical ecosystems

doi:10.1002/2013GC005015

CORC > 北京大学 > 环境科学与工程学院

	Comparable hydrogen isotopic fractionation of plant leaf wax n-alkanoic acids in arid and humid subtropical ecosystems
	Gao, Li ; Zheng, Mei ; Fraser, Matthew ; Huang, Yongsong
刊名	geochemistry geophysics geosystems
	2014
关键词	leaf waxes hydrogen isotope fractionation ecosystems comparable arid humid DELTA-D VALUES STABLE CARBON D/H RATIOS ATMOSPHERIC AEROSOLS LIPID BIOMARKERS SURFACE SEDIMENT LAKE-SEDIMENTS RECORD CLIMATE TERRESTRIAL
DOI	10.1002/2013GC005015
英文摘要	Leaf wax hydrogen isotope proxies have been widely used to reconstruct past hydrological changes. However, published reconstructions have given little consideration for the potentially variable hydrogen isotopic fractionation relative to precipitation (epsilon wax-p) under different climate and environmental settings. Chief among various potential factors controlling fractionation is relative humidity, which is known to strongly affect oxygen isotopic ratios of plant cellulose, but its effect on hydrogen isotopic fractionation of leaf waxes is still ambiguous. Analyses of lake surface sediments and individual modern plants have provided valuable information on the variability of epsilon wax-p, but both approaches have significant limitations. Here, we present an alternative method to obtain the integrated, time-resolved ecosystem-level epsilon wax-p values, by analyzing modern aerosol samples collected weekly from arid (Arizona lowlands) and humid subtropical (Atlanta, Georgia) environments during the main growth season. Because aerosol samples mainly reflect regional leaf wax resources, the extreme contrast in the hydroclimate and associated vegetation assemblages between our study sites allows us to rigorously assess the impact of relative humidity and associated vegetation assemblages on leaf wax hydrogen isotopic fractionation. We show there is only minor difference (mostly <10 parts per thousand) in the mean epsilon wax-p values in the two end-member environments. One possible explanation is that the positive isotopic effects of low relative humidity are offset by progressive replacement of trees with grasses that have a more negative apparent fractionation. Our results represent an important step toward quantitative interpretation of leaf wax hydrogen isotopic records.; Geochemistry & Geophysics; SCI(E); EI; 3; ARTICLE; yongsong_huang@brown.edu; 2; 361-373; 15
语种	英语
内容类型	期刊论文
源URL	[http://ir.pku.edu.cn/handle/20.500.11897/216952]
专题	环境科学与工程学院
推荐引用方式 GB/T 7714	Gao, Li,Zheng, Mei,Fraser, Matthew,et al. Comparable hydrogen isotopic fractionation of plant leaf wax n-alkanoic acids in arid and humid subtropical ecosystems[J]. geochemistry geophysics geosystems,2014.
APA	Gao, Li,Zheng, Mei,Fraser, Matthew,&Huang, Yongsong.(2014).Comparable hydrogen isotopic fractionation of plant leaf wax n-alkanoic acids in arid and humid subtropical ecosystems.geochemistry geophysics geosystems.
MLA	Gao, Li,et al."Comparable hydrogen isotopic fractionation of plant leaf wax n-alkanoic acids in arid and humid subtropical ecosystems".geochemistry geophysics geosystems (2014).