An Alkane-Soluble Dendrimer as Electron-Transport Layer in Polymer Light-Emitting Diodes | |
Zhong, Zhiming ; Zhao, Sen ; Pei, Jian ; Wang, Jian ; Ying, Lei ; Peng, Junbiao ; Cao, Yong | |
刊名 | ACS APPLIED MATERIALS & INTERFACES |
2016 | |
关键词 | polymer light-emitting diodes solution process multilayer device alkane soluble electron transport FIELD-EFFECT TRANSISTORS SOLAR-CELLS HIGHLY EFFICIENT CONJUGATED POLYMERS DEVICE PERFORMANCE SOLVENT TREATMENT INJECTION LAYER RED BLUE COPOLYMERS |
DOI | 10.1021/acsami.6b05172 |
英文摘要 | Polymer light-emitting diodes (PLEDs) have attracted broad interest due to their solution-processable properties. It is well-known that to achieve better performance, organic light-emitting diodes require multilayer device structures. However, it is difficult to realize multilayer device structures by solution processing for PLEDs. Because most semiconducting polymers have similar solubility in common organic solvents, such as toluene, xylene, chloroform, and chlorobenzene, the deposition of multilayers can cause layers to mix together and damage each layer. Herein, a novel semiorthogonal solubility relationship was developed and demonstrated. For the first time, an alkane-soluble dendrimer is utilized as the electron-transport layer (ETL) in PLEDs via a solution-based process. With the dendrimer ETL, the external quantum efficiency increases more than threefold. This improvement in the device performance is attributed to better exciton confinement, improved exciton energy transfer, and better charge carrier balance. The semiorthogonal solubility provided by alkane offers another process dimension in PLEDs. By combining them with water/alcohol-soluble polyelectrolytes, more exquisite multilayer devices can be fabricated to achieve high device performance, and new device structures can be designed and realized.; Ministry of Science and Technology (973 Program) [2015CB655000]; National Nature Science Foundation of China [51573056, 51373057]; Integration of Production and Research Projects of Guangdong Province [2014B090916001, 2015B090915001]; SCI(E); EI; PubMed; ARTICLE; jianwang@scut.edu.cn; msleiying@scut.edu.cn; 31; 20238-20243; 8 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/491614] |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Zhong, Zhiming,Zhao, Sen,Pei, Jian,et al. An Alkane-Soluble Dendrimer as Electron-Transport Layer in Polymer Light-Emitting Diodes[J]. ACS APPLIED MATERIALS & INTERFACES,2016. |
APA | Zhong, Zhiming.,Zhao, Sen.,Pei, Jian.,Wang, Jian.,Ying, Lei.,...&Cao, Yong.(2016).An Alkane-Soluble Dendrimer as Electron-Transport Layer in Polymer Light-Emitting Diodes.ACS APPLIED MATERIALS & INTERFACES. |
MLA | Zhong, Zhiming,et al."An Alkane-Soluble Dendrimer as Electron-Transport Layer in Polymer Light-Emitting Diodes".ACS APPLIED MATERIALS & INTERFACES (2016). |
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