Spin Manipulation by Creation of Single-Molecule Radical Cations | |
Karan, Sujoy ; Li, Na ; Zhang, Yajie ; He, Yang ; Hong, I-Po ; Song, Huanjun ; Lu, Jing-Tao ; Wang, Yongfeng ; Peng, Lianmao ; Wu, Kai ; Michelitsch, Georg S. ; Maurer, Reinhard J. ; Diller, Katharina ; Reuter, Karsten ; Weismann, Alexander ; Berndt, Richard | |
刊名 | PHYSICAL REVIEW LETTERS
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2016 | |
关键词 | KONDO RESONANCE MAGNETIC IMPURITY METAL-SURFACES RETINOIC ACID MODEL ATOM SPINTRONICS ADSORPTION FIELD |
DOI | 10.1103/PhysRevLett.116.027201 |
英文摘要 | All-trans-retinoic acid (ReA), a closed-shell organic molecule comprising only C, H, and O atoms, is investigated on a Au(111) substrate using scanning tunneling microscopy and spectroscopy. In dense arrays single ReA molecules are switched to a number of states, three of which carry a localized spin as evidenced by conductance spectroscopy in high magnetic fields. The spin of a single molecule may be reversibly switched on and off without affecting its neighbors. We suggest that ReA on Au is readily converted to a radical by the abstraction of an electron.; Deutsche Forschungsgemeinschaft (DFG) [SFB 677]; National Natural Science Foundation of China [21522301, 21373020, 21403008, 61321001, 21433011, 21333001]; Ministry of Science and Technology [2014CB239302, 2013CB933400]; Research Fund for the Doctoral Program of Higher Education [20130001110029]; DFG; Gauss Centre for Supercomputing/Leibniz Supercomputing Centre [pr94sa]; SCI(E); EI; PubMed; ARTICLE; yongfengwang@pku.edu.cn; berndt@physik.uni-kiel.de; 2; 027201; 116 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/435161] ![]() |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Karan, Sujoy,Li, Na,Zhang, Yajie,et al. Spin Manipulation by Creation of Single-Molecule Radical Cations[J]. PHYSICAL REVIEW LETTERS,2016. |
APA | Karan, Sujoy.,Li, Na.,Zhang, Yajie.,He, Yang.,Hong, I-Po.,...&Berndt, Richard.(2016).Spin Manipulation by Creation of Single-Molecule Radical Cations.PHYSICAL REVIEW LETTERS. |
MLA | Karan, Sujoy,et al."Spin Manipulation by Creation of Single-Molecule Radical Cations".PHYSICAL REVIEW LETTERS (2016). |
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