Multiple-timescale relaxation dynamics in CsGd(MoO4)(2)-a dipolar magnet with a highly anisotropic layered crystal structure | |
Tkac, V. ; Orendacova, A. ; Tarasenko, R. ; Cizmar, E. ; Orendac, M. ; Tibenska, K. ; Anders, A. G. ; Gao, S. ; Pavlik, V. ; Feher, A. | |
刊名 | journal of physics condensed matter |
2013 | |
关键词 | SPIN-LATTICE RELAXATION RARE-EARTH MOLYBDATES PARAMAGNETIC RELAXATION THERMAL-CONDUCTIVITY SOUND-ATTENUATION EXPONENTS |
DOI | 10.1088/0953-8984/25/50/506001 |
英文摘要 | The dynamic properties of the dipolar magnet CsGd(MoO4)(2) have been studied. The frequency and temperature dependence of the AC susceptibility investigated in the paramagnetic region above 2 K revealed the co-existence of magnetic field induced slow and fast relaxation channels with a timescale differing by three orders of magnitude. The slow relaxation is determined by the properties of the first coordination sphere of the Gd3+ C ion and has the character of a two-phonon Orbach process. The fast relaxation is potentially attributed to a two-phonon Raman process realized via a localized phonon mode associated with the layered crystal structure. The temperature dependence of the phonon mean free path in zero magnetic field indicates significant phonon scattering below 1 K resulting from the combined effect of magnetic correlations and the scattering of dominant phonons with energies corresponding to the crystal-field levels.; Physics, Condensed Matter; SCI(E); EI; 0; ARTICLE; 50; 25 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/390750] |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Tkac, V.,Orendacova, A.,Tarasenko, R.,et al. Multiple-timescale relaxation dynamics in CsGd(MoO4)(2)-a dipolar magnet with a highly anisotropic layered crystal structure[J]. journal of physics condensed matter,2013. |
APA | Tkac, V..,Orendacova, A..,Tarasenko, R..,Cizmar, E..,Orendac, M..,...&Feher, A..(2013).Multiple-timescale relaxation dynamics in CsGd(MoO4)(2)-a dipolar magnet with a highly anisotropic layered crystal structure.journal of physics condensed matter. |
MLA | Tkac, V.,et al."Multiple-timescale relaxation dynamics in CsGd(MoO4)(2)-a dipolar magnet with a highly anisotropic layered crystal structure".journal of physics condensed matter (2013). |
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