Multifunctional photoelectrochemical logic gates based on a hemicyanine sensitized semiconductor electrode | |
Li, FY ; Shi, M ; Huang, CH ; Jin, LP | |
刊名 | 材料化学杂志 |
2005 | |
关键词 | LANGMUIR-BLODGETT-FILMS LB MONOLAYER FILMS MOLECULAR LOGIC 2ND-HARMONIC GENERATION PHOTOCURRENT GENERATION ITO ELECTRODES HETERO-FILM DYE CONVERSION FLUORESCENCE |
DOI | 10.1039/b502692j |
英文摘要 | A new amphiphilic hemicyanine dye, (E)-1,3,3-trimethyl-2-[2-( 4-N-methyl-N-hexadecylaminophenyl)ethenyl] indolinium iodide(MHID) has been synthesized and successfully transferred onto a semiconducting transparent indium-tin oxide (ITO) electrode by Langmuir-Blodgett (LB) techniques. The photoelectric conversion properties of the dye MHID monolayer fabricated ITO electrode have been investigated in a three electrode photoelectrochemical cell. The observed photocurrent strongly depends on the applied electrode potential and the concentrations of the electron acceptors and donors. By using electron acceptors and (or) donors as input and photocurrent as output, respectively, we have fabricated this artificial photoelectrochemical system as multifunctional logic gates, corresponding to a series of logic operations (YES, OR, XOR and INHIBIT). Importantly, the gates of this photoelectrochemical system have been interconnected to demonstrate computation as a half-subtractor, with Eu3+ and hydroquinone (H(2)Q) as the two inputs and the cathodic photocurrent and the absolute value of the photocurrent as the two outputs, respectively.; Chemistry, Physical; Materials Science, Multidisciplinary; SCI(E); EI; 22; ARTICLE; 29; 3015-3020; 15 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/254188] |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Li, FY,Shi, M,Huang, CH,et al. Multifunctional photoelectrochemical logic gates based on a hemicyanine sensitized semiconductor electrode[J]. 材料化学杂志,2005. |
APA | Li, FY,Shi, M,Huang, CH,&Jin, LP.(2005).Multifunctional photoelectrochemical logic gates based on a hemicyanine sensitized semiconductor electrode.材料化学杂志. |
MLA | Li, FY,et al."Multifunctional photoelectrochemical logic gates based on a hemicyanine sensitized semiconductor electrode".材料化学杂志 (2005). |
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