Thermochemical hole burning on a series of N-substituted morpholinium 7,7,8,8-tetracyanoquinodimethane charge-transfer complexes for data storage | |
Ran, CB ; Peng, HL ; Zhou, W ; Yu, XC ; Liu, ZF | |
刊名 | journal of physical chemistry b
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2005 | |
关键词 | SCANNING-TUNNELING-MICROSCOPY ATOMIC-FORCE MICROSCOPE DENSITY DATA-STORAGE NANOMETER-SCALE THIN-FILMS TRANSITIONS SURFACE TIPS |
DOI | 10.1021/jp0528616 |
英文摘要 | We demonstrate here the thermochemical hole burning (THB) effect on a series of N-substituted morpholinium 7,7,8,8-tetracyanoquinodimethane charge-transfer (C-T) complexes for ultra-high-density data storage. A correlation between the decomposition temperature of the charge-transfer complex and the threshold voltage of hole burning was observed: the higher the decomposition temperature, the larger the writing threshold value, suggesting the possibility of molecular design for optimizing the hole burning performance. The macroscopic decomposition properties of these charge-transfer complexes were studied by thermal gravimetry combined with mass spectrometry. Theoretical estimation of the temperature rise induced by scanning tunneling microscopy current heating was also conducted, which indicated that the maximum temperature certainly exceeds the decomposition temperatures of these C-T complexes. These observations are consistent with the thermochernical hole burning mechanism.; Chemistry, Physical; SCI(E); PubMed; 15; ARTICLE; 47; 22486-22490; 109 |
语种 | 英语 |
内容类型 | 期刊论文 |
源URL | [http://ir.pku.edu.cn/handle/20.500.11897/198745] ![]() |
专题 | 化学与分子工程学院 |
推荐引用方式 GB/T 7714 | Ran, CB,Peng, HL,Zhou, W,et al. Thermochemical hole burning on a series of N-substituted morpholinium 7,7,8,8-tetracyanoquinodimethane charge-transfer complexes for data storage[J]. journal of physical chemistry b,2005. |
APA | Ran, CB,Peng, HL,Zhou, W,Yu, XC,&Liu, ZF.(2005).Thermochemical hole burning on a series of N-substituted morpholinium 7,7,8,8-tetracyanoquinodimethane charge-transfer complexes for data storage.journal of physical chemistry b. |
MLA | Ran, CB,et al."Thermochemical hole burning on a series of N-substituted morpholinium 7,7,8,8-tetracyanoquinodimethane charge-transfer complexes for data storage".journal of physical chemistry b (2005). |
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