Hierarchical quantum master equation with semiclassical Drude dissipation

doi:10.1063/1.3268922

CORC > 化学研究所 > 中国科学院化学研究所

	Hierarchical quantum master equation with semiclassical Drude dissipation
	Xu, Rui-Xue 1,2; Tian, Bao-Ling 1,2; Xu, Jian 1,2; Shi, Qiang 3; Yan, YiJing 2
刊名	JOURNAL OF CHEMICAL PHYSICS
	2009-12-07
卷号	131 期号:21
ISSN号	0021-9606
DOI	10.1063/1.3268922
英文摘要	We propose a nonperturbative quantum dissipation theory, in term of hierarchical quantum master equation, which may be used with a great degree of confidence to various dynamics systems in condensed phases. The theoretical development is rooted in an improved semiclassical treatment of Drude bath, beyond the conventional high temperature approximations. It leads to the new theory a simple but important improvement over the conventional stochastic Liouville equation theory, without extra numerical cost. Its broad range of validity and applicability is extensively demonstrated with two-level electron transfer model systems, where the new theory can be considered as the modified Zusman equation. Criterion is also proposed to estimate the performance of the hierarchical quantum master equation. (C) 2009 American Institute of Physics. [doi: 10.1063/1.3268922]
语种	英语
出版者	AMER INST PHYSICS
WOS记录号	WOS:000272494300013
内容类型	期刊论文
源URL	[http://ir.iccas.ac.cn/handle/121111/66991]
专题	中国科学院化学研究所
通讯作者	Xu, Rui-Xue
作者单位	1.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China 2.Hong Kong Univ Sci & Technol, Dept Chem, Kowloon, Hong Kong, Peoples R China 3.Chinese Acad Sci, Inst Chem, Beijing Natl Lab Mol Sci, State Key Lab Struct Chem Unstable & Stable Speci, Beijing 100190, Peoples R China
推荐引用方式 GB/T 7714	Xu, Rui-Xue,Tian, Bao-Ling,Xu, Jian,et al. Hierarchical quantum master equation with semiclassical Drude dissipation[J]. JOURNAL OF CHEMICAL PHYSICS,2009,131(21).
APA	Xu, Rui-Xue,Tian, Bao-Ling,Xu, Jian,Shi, Qiang,&Yan, YiJing.(2009).Hierarchical quantum master equation with semiclassical Drude dissipation.JOURNAL OF CHEMICAL PHYSICS,131(21).
MLA	Xu, Rui-Xue,et al."Hierarchical quantum master equation with semiclassical Drude dissipation".JOURNAL OF CHEMICAL PHYSICS 131.21(2009).