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Determination of the effective diffusion coefficient for 125I(-) in Beishan granite
Lu, C. J.1; Liu, C. L.1; Chen, T.1; Wang, J.2; Wang, X. Y.1; Su, R.2; Sun, J. Y.1; Yang, R. X.1; Zhang, X. S.1
刊名RADIOCHIMICA ACTA
2008
卷号96期号:2页码:111-117
关键词Effective Diffusion Coefficient I-125(-) Beishan Granite Geological Disposal High-level Radioactive Wastes
ISSN号0033-8230
DOI10.1524/ract.2008.1469
英文摘要With the policy of active development of nuclear energy in China in the following 20 years or more, the high-level radioactive wastes and spent fuels will increase considerably. In order to dispose of these wastes safely, China plans to construct a geological repository in the middle of the 21st century. Through more than 20 years of research and discussion in China, granite has been regarded as one of the most favorable candidate host rocks for a potential geological repository and I-129 has been recognized as one of the most important nuclides for the safety of the potential repository. In this paper, the diffusion of I-125 (as a surrogate of I-129) in deep granite taken from Beishan, Gansu Province is investigated with the help of a small scale diffusion apparatus. The granite core sample was taken at the depth of about 300 m and cut into sections of 5 similar to 20 mm. The granite section samples were weighted and the pore volume was determined with water immersion method. The chemical and elemental compositions of the granite are presented. Experimental results were treated with different methods, producing an effective diffusion coefficient of I-125(-) in the granite of (2.44-2.72) x 10(-12) m(2) s(-1).
语种英语
出版者OLDENBOURG VERLAG
WOS记录号WOS:000253497100007
内容类型期刊论文
源URL[http://ir.iccas.ac.cn/handle/121111/65615]  
专题中国科学院化学研究所
通讯作者Liu, C. L.
作者单位1.Peking Univ, Coll Chem & Mol Engn, Dept Appl Chem, Beijing Natl Lab Mol Sci, Beijing 100871, Peoples R China
2.China Natl Nucl Corp, Beijing Res Inst Uranium Geol, Beijing 100029, Peoples R China
推荐引用方式
GB/T 7714
Lu, C. J.,Liu, C. L.,Chen, T.,et al. Determination of the effective diffusion coefficient for 125I(-) in Beishan granite[J]. RADIOCHIMICA ACTA,2008,96(2):111-117.
APA Lu, C. J..,Liu, C. L..,Chen, T..,Wang, J..,Wang, X. Y..,...&Zhang, X. S..(2008).Determination of the effective diffusion coefficient for 125I(-) in Beishan granite.RADIOCHIMICA ACTA,96(2),111-117.
MLA Lu, C. J.,et al."Determination of the effective diffusion coefficient for 125I(-) in Beishan granite".RADIOCHIMICA ACTA 96.2(2008):111-117.
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