Visible-Light Photocatalytic Degradation of Methylene Blue Using SnO2/-Fe2O3 Hierarchical Nanoheterostructures | |
Zhang, Shouwei1,2; Li, Jiaxing1; Niu, Haihong2; Xu, Wenqing3; Xu, Jinzhang2; Hu, Wenping4; Wang, Xiangke1 | |
刊名 | CHEMPLUSCHEM |
2013-02-01 | |
卷号 | 78期号:2页码:192-199 |
关键词 | Charge Separation Environmental Chemistry Nanostructures Photocatalysis Sno2 -fe2o3 Visible Light |
ISSN号 | 2192-6506 |
DOI | 10.1002/cplu.201200272 |
英文摘要 | Three-dimensional SnO2/-Fe2O3 semiconductor hierarchical nanoheterostructures were synthesized for photocatalysis through a low-cost and environmentally friendly hydrothermal strategy, by crystallographic-oriented epitaxial growth of SnO2 on three-dimensional -Fe2O3 flowerlike hierarchical nanostructures. In this photocatalyst, visible-light-active Fe2O3 flowerlike hierarchical nanostructures were used as a medium to absorb photons and convert them into photogenerated charges, and SnO2 nanoparticles were used as charge collectors to transport the photogenerated charges. The SnO2/-Fe2O3 semiconductor hierarchical nanoheterostructures exhibited excellent visible-light photocatalytic ability for the degradation of methylene blue; this was attributed to the large specific surface area, wide visible-light absorption range, and efficient electronhole pair separation properties of the SnO2/-Fe2O3 nanoheterostructures. The SnO2/-Fe2O3 material showed improved separation of photogenerated electronhole pairs owing to the potential-energy differences between SnO2 and -Fe2O3, and therefore exhibited enhanced photocatalytic activity. This paper highlights the SnO2/-Fe2O3 semiconductor hierarchical nanoheterostructures as potentially more environmentally friendly materials for use in organic pollutant degradation for environmental pollution cleanup operations. |
语种 | 英语 |
出版者 | WILEY-V C H VERLAG GMBH |
WOS记录号 | WOS:000315117100009 |
内容类型 | 期刊论文 |
源URL | [http://ir.iccas.ac.cn/handle/121111/54363] |
专题 | 中国科学院化学研究所 |
通讯作者 | Wang, Xiangke |
作者单位 | 1.Chinese Acad Sci, Inst Plasma Phys, Key Lab Novel Thin Film Solar Cells, Hefei 230031, Peoples R China 2.Hefei Univ Technol, Sch Mat Sci & Engn, Hefei 230031, Peoples R China 3.Yale Univ, Dept Chem Engn, Environm Engn Program, New Haven, CT 06520 USA 4.Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Shouwei,Li, Jiaxing,Niu, Haihong,et al. Visible-Light Photocatalytic Degradation of Methylene Blue Using SnO2/-Fe2O3 Hierarchical Nanoheterostructures[J]. CHEMPLUSCHEM,2013,78(2):192-199. |
APA | Zhang, Shouwei.,Li, Jiaxing.,Niu, Haihong.,Xu, Wenqing.,Xu, Jinzhang.,...&Wang, Xiangke.(2013).Visible-Light Photocatalytic Degradation of Methylene Blue Using SnO2/-Fe2O3 Hierarchical Nanoheterostructures.CHEMPLUSCHEM,78(2),192-199. |
MLA | Zhang, Shouwei,et al."Visible-Light Photocatalytic Degradation of Methylene Blue Using SnO2/-Fe2O3 Hierarchical Nanoheterostructures".CHEMPLUSCHEM 78.2(2013):192-199. |
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