The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)

doi:10.1134/S0036024417020352

	The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)
	Lu, Xingqiang 3; Guo, Wei 1,2; Wang, Xinlin 1
刊名	RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A
	2017
卷号	91 期号:2 页码:366-372
关键词	Photoelectron Spectra State Populations Time-dependent Wave Packet Approach Three-level Ladder K-2 Molecule
ISSN号	0036-0244
DOI	10.1134/S0036024417020352
文献子类	Article
英文摘要	The delay time dependence of photoelectron spectra and state populations of three-level ladder K-2 molecule is investigated by pump-probe pulses via time-dependent wave packet approach. The periodical motion of the wave packet with oscillating period 500 fs results in the periodical variation of photoelectron spectra. The photoelectron spectra show Autler-Townes double splitting at zero delay time, and no splitting at positive delay time. The periodical change of state populations with delay time can be ascribed to the coupling effect between the two pulses. It is found that the selectivity of the state populations may be attained by regulating the delay time. The results can provide some important basis for realizing the optical control of molecules experimentally.
WOS关键词	PROBE FEMTOSECOND SPECTROSCOPY ; ULTRASHORT LASER-PULSES ; WAVE-PACKET DYNAMICS ; ELECTRONIC STATES ; NA-2 MOLECULE ; EXCITED-STATES ; PHOTODISSOCIATION ; WAVEPACKET ; FIELDS ; NAK
WOS研究方向	Chemistry
语种	英语
出版者	MAIK NAUKA/INTERPERIODICA/SPRINGER
WOS记录号	WOS:000395076500031
内容类型	期刊论文
源URL	[http://cas-ir.dicp.ac.cn/handle/321008/169564]
专题	大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者	Lu, Xingqiang
作者单位	1.Univ South China, Sch Elect Engn, Hengyang 421001, Peoples R China 2.Dalian Inst Chem Phys, State Key Lab Mol React Dynam, Dalian 116023, Peoples R China 3.Univ South China, Sch Nucl Sci & Technol, Hengyang 421001, Peoples R China
推荐引用方式 GB/T 7714	Lu, Xingqiang,Guo, Wei,Wang, Xinlin. The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)[J]. RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A,2017,91(2):366-372.
APA	Lu, Xingqiang,Guo, Wei,&Wang, Xinlin.(2017).The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1).RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A,91(2),366-372.
MLA	Lu, Xingqiang,et al."The Delay Time Dependence of the Photoelectron Spectra and State Populations of Three-Level Ladder K-2 Molecule(1)".RUSSIAN JOURNAL OF PHYSICAL CHEMISTRY A 91.2(2017):366-372.