Growth of Cu/SSZ-13 on SiC for selective catalytic reduction of NO with NH3
Zhou, Tiaoyun2,3,4,5; Pan, Xiulian3; Bao, Xinhe3; Yuan, Qing1,3
刊名CHINESE JOURNAL OF CATALYSIS
2018-01-18
卷号39期号:1页码:71-78
关键词Zeolite Ssz-13 Silicon Carbide Selective Catalytic Reduction By Ammonia
ISSN号1872-2067
DOI10.1016/S1872-2067(17)62870-5
文献子类Article
英文摘要Silicon carbide (SiC) was used as a support for SSZ-13 zeolite in an attempt to improve the high-temperature stability and activity of Cu/SSZ-13 in the selective catalytic reduction (SCR) of NO with NH3. SSZ-13 was grown via a hydrothermal method using the silicon and silica contained in SiC as the source of silicon, which led to the formation of a chemically bonded SSZ-13 layer on SiC. Characterization using X-ray diffraction, scanning electron microscopy, and N-2 adsorption-desorption isotherms revealed that the alkali content strongly affected the purity of zeolite and the crystallization time affected the coverage and crystallinity of the zeolite layer. Upon ion exchange, the resulting Cu/SSZ-13@SiC catalyst exhibited enhanced activity in NH3-SCR in the high-temperature region compared with the unsupported Cu/SSZ-13. Thus, the application temperature was extended with the use of SiC as the support. (C) 2018, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
WOS关键词SILICON-CARBIDE ; NITRIC-OXIDE ; ZEOLITE ; AMMONIA ; SCR ; DEACTIVATION ; HYDROGEN ; AG/AL2O3 ; SUPPORT ; SAPO-34
WOS研究方向Chemistry ; Engineering
语种英语
出版者SCIENCE PRESS
WOS记录号WOS:000428822100010
内容类型期刊论文
源URL[http://cas-ir.dicp.ac.cn/handle/321008/169168]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Pan, Xiulian; Bao, Xinhe
作者单位1.Dalian Nationalities Univ, Sch Phys & Mat Engn, Key Lab New Energy & Rare Earth Resource Utilizat, State Ethn Affairs Commiss, Dalian 116600, Liaoning, Peoples R China
2.Chinese Acad Sci, Shanghai Adv Res Inst, Shanghai 201210, Peoples R China
3.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
5.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
推荐引用方式
GB/T 7714
Zhou, Tiaoyun,Pan, Xiulian,Bao, Xinhe,et al. Growth of Cu/SSZ-13 on SiC for selective catalytic reduction of NO with NH3[J]. CHINESE JOURNAL OF CATALYSIS,2018,39(1):71-78.
APA Zhou, Tiaoyun,Pan, Xiulian,Bao, Xinhe,&Yuan, Qing.(2018).Growth of Cu/SSZ-13 on SiC for selective catalytic reduction of NO with NH3.CHINESE JOURNAL OF CATALYSIS,39(1),71-78.
MLA Zhou, Tiaoyun,et al."Growth of Cu/SSZ-13 on SiC for selective catalytic reduction of NO with NH3".CHINESE JOURNAL OF CATALYSIS 39.1(2018):71-78.
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