Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon
Cui, Tingting1,2; Bao, Xinhe2; Lin, Yaping1,2; Li, Pan2; Pan, Xiulian2
刊名JOURNAL OF ENERGY CHEMISTRY
2018-05-01
卷号27期号:3页码:898-902
关键词Co Methanation Ni Catalyst Carbon Nitrogen Doping Sic
ISSN号2095-4956
DOI10.1016/j.jechem.2017.06.008
文献子类Article
英文摘要Nitrogen doping has been proved to be an effective way to modify the properties of graphene and other carbon materials. Herein, we explore a composite with nitrogen doped carbon overlayers wrapping SiC substrate as a support for Ni (Ni/CN-SiC) and evaluate its effects on the methanation activity. The results show that both the activity and stability of Ni are enhanced. Characterization with STEM, XRD, XPS, Raman and H-2 - TPR indicates that nitrogen doping generates more defects in the carbon overlayers, which benefit the dispersion of Ni. Furthermore, the reduction of Ni is facilitated. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved.
WOS关键词FISCHER-TROPSCH SYNTHESIS ; SYNTHETIC NATURAL-GAS ; OXYGEN REDUCTION ; IRON CATALYSTS ; GRAPHENE ; PERFORMANCE ; 1ST-PRINCIPLE ; HYDROGENATION ; NANOTUBES ; NI(111)
WOS研究方向Chemistry ; Energy & Fuels ; Engineering
语种英语
出版者ELSEVIER SCIENCE BV
WOS记录号WOS:000430515900032
内容类型期刊论文
源URL[http://cas-ir.dicp.ac.cn/handle/321008/169142]  
专题大连化学物理研究所_中国科学院大连化学物理研究所
通讯作者Bao, Xinhe; Pan, Xiulian
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China
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GB/T 7714
Cui, Tingting,Bao, Xinhe,Lin, Yaping,et al. Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon[J]. JOURNAL OF ENERGY CHEMISTRY,2018,27(3):898-902.
APA Cui, Tingting,Bao, Xinhe,Lin, Yaping,Li, Pan,&Pan, Xiulian.(2018).Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon.JOURNAL OF ENERGY CHEMISTRY,27(3),898-902.
MLA Cui, Tingting,et al."Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon".JOURNAL OF ENERGY CHEMISTRY 27.3(2018):898-902.
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