Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon | |
Cui, Tingting1,2; Bao, Xinhe2; Lin, Yaping1,2; Li, Pan2; Pan, Xiulian2 | |
刊名 | JOURNAL OF ENERGY CHEMISTRY
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2018-05-01 | |
卷号 | 27期号:3页码:898-902 |
关键词 | Co Methanation Ni Catalyst Carbon Nitrogen Doping Sic |
ISSN号 | 2095-4956 |
DOI | 10.1016/j.jechem.2017.06.008 |
文献子类 | Article |
英文摘要 | Nitrogen doping has been proved to be an effective way to modify the properties of graphene and other carbon materials. Herein, we explore a composite with nitrogen doped carbon overlayers wrapping SiC substrate as a support for Ni (Ni/CN-SiC) and evaluate its effects on the methanation activity. The results show that both the activity and stability of Ni are enhanced. Characterization with STEM, XRD, XPS, Raman and H-2 - TPR indicates that nitrogen doping generates more defects in the carbon overlayers, which benefit the dispersion of Ni. Furthermore, the reduction of Ni is facilitated. (C) 2017 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. and Science Press. All rights reserved. |
WOS关键词 | FISCHER-TROPSCH SYNTHESIS ; SYNTHETIC NATURAL-GAS ; OXYGEN REDUCTION ; IRON CATALYSTS ; GRAPHENE ; PERFORMANCE ; 1ST-PRINCIPLE ; HYDROGENATION ; NANOTUBES ; NI(111) |
WOS研究方向 | Chemistry ; Energy & Fuels ; Engineering |
语种 | 英语 |
出版者 | ELSEVIER SCIENCE BV |
WOS记录号 | WOS:000430515900032 |
内容类型 | 期刊论文 |
源URL | [http://cas-ir.dicp.ac.cn/handle/321008/169142] ![]() |
专题 | 大连化学物理研究所_中国科学院大连化学物理研究所 |
通讯作者 | Bao, Xinhe; Pan, Xiulian |
作者单位 | 1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 2.Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Liaoning, Peoples R China |
推荐引用方式 GB/T 7714 | Cui, Tingting,Bao, Xinhe,Lin, Yaping,et al. Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon[J]. JOURNAL OF ENERGY CHEMISTRY,2018,27(3):898-902. |
APA | Cui, Tingting,Bao, Xinhe,Lin, Yaping,Li, Pan,&Pan, Xiulian.(2018).Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon.JOURNAL OF ENERGY CHEMISTRY,27(3),898-902. |
MLA | Cui, Tingting,et al."Modulating the CO methanation activity of Ni catalyst by nitrogen doped carbon".JOURNAL OF ENERGY CHEMISTRY 27.3(2018):898-902. |
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